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High-resolution dissociative recombination of cold H3+and first evidence for nuclear spin effects
Authors:Kreckel H  Motsch M  Mikosch J  Glosík J  Plasil R  Altevogt S  Andrianarijaona V  Buhr H  Hoffmann J  Lammich L  Lestinsky M  Nevo I  Novotny S  Orlov D A  Pedersen H B  Sprenger F  Terekhov A S  Toker J  Wester R  Gerlich D  Schwalm D  Wolf A  Zajfman D
Affiliation:Max-Planck-Institut für Kernphysik, Heidelberg, Germany.
Abstract:The energy-resolved rate coefficient for the dissociative recombination (DR) of H(3)(+) with slow electrons has been measured by the storage-ring method using an ion beam produced from a radiofrequency multipole ion trap, employing buffer-gas cooling at 13 K. The electron energy spread of the merged-beams measurement is reduced to 500 microeV by using a cryogenic GaAs photocathode. This and a previous cold- measurement jointly confirm the capability of ion storage rings, with suitable ion sources, to store and investigate H(3)(+) in the two lowest, (J,G) = (1,1) and (1,0) rotational states prevailing also in cold interstellar matter. The use of para-H(2) in the ion source, expected to enhance para-H(3)(+) in the stored ion beam, is found to increase the DR rate coefficient at meV electron energies.
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