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ESR of double-perovskite Sr2FeMoO6
Authors:M T Causa  A Butera  M Tovar  J Fontcuberta
Institution:

a Centro Atómico Bariloche, Comisión Nacional de Energía Atómica and Instituto Balseiro, Universidad Nacional de Cuyo, 8400 Bariloche, Río Negro, Argentina

b Institut de Ciència de Materials de Barcelona, Consejo Superior de Investigación Científica, E-08193 Bellaterra, Catalunya, Spain

Abstract:We present an ESR study of Sr2FeMoO6 in the paramagnetic region. A single line at g≈2 was associated with Fe3+ ions. The intensity follows Curie–Weiss law in the whole T range. For T >500 K a secondary line is attributed to ferromagnetic (FM) impurities. The line width is described by ΔHpp(T)=ΔHpp(∞)(1?Θ/T) with a high value for ΔHpp(∞). The absence of narrowing effects is a signature of double-exchange (DE) interactions and indicates that DE drives the FM ordering at a relatively high Tc.
Keywords:Double exchange  Magnetoresistant materials  ESR
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