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X-ray magnetic circular dichroism measurements in Ni up to 200 GPa: resistant ferromagnetism
Authors:Torchio R  Kvashnin Y O  Pascarelli S  Mathon O  Marini C  Genovese L  Bruno P  Garbarino G  Dewaele A  Occelli F  Loubeyre P
Institution:European Synchrotron Radiation Facility, 6 Rue Jules Horowitz, BP220, 38043 Grenoble Cedex, France.
Abstract:The structural stability of fcc Ni over a very large pressure range offers a unique opportunity to experimentally investigate how magnetism is modified by simple compression. K-edge x-ray magnetic circular dichroism (XMCD) shows that fcc Ni is ferromagnetic up to 200 GPa, contradicting recent predictions of an abrupt transition to a paramagnetic state at 160 GPa. Density functional theory calculations point out that the pressure evolution of the K-edge XMCD closely follows that of the p projected orbital moment rather than that of the total spin moment. The disappearance of magnetism in Ni is predicted to occur above 400 GPa.
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