Theory of resonance hyper-Raman induced by realistic coherent pulses |
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| Authors: | T. Ben-Zeev A.D. Wilson H. Friedmann |
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| Affiliation: | Department of Chemistry, Bar-Ilan University, Ramat-Gan, Israel |
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| Abstract: | We present a theory of time-resolved and frequency-resolved resonance hyper-Raman induced by realistic, coherent, quasi-rectangular pulses. In particular, we treat the case where the mean frequency ω of the incident pulse is in near-resonance with the molecular transition frequency ωmn. New peaks are predicted and saturation effects are discussed. |
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