Plume separation effect in pulsed laser ablation deposition

The results of a new geometrical configuration of pulsed laser ablation deposition technique that uses a hemi-cylindrical transparent plastic substrate are presented and discussed. With the new arrangement, two distinct components with different material compositions have been clearly observed. While the first component comprises atoms, ions and molecules and constitutes visible or the so-called luminous plume, the second component is formed of fragments, clusters and liquid droplets and is invisible to the naked eye. The latter component constitutes a major part of the ablated material. The luminous plume symmetry axis does not coincide with the mass distribution symmetry axis. In the case of Si ablation and 45° incident beam angle, the maximum deflection angle of the luminous plume reaches 30° with respect to the normal to the target surface, while the deflection angle of the second component is higher than 40°. The change in the target morphology and the dependence of the composition of the ablated material on local fluence, along with the hydrodynamic effects, is sought to explain this previously unexpected and unreported phenomenon. PACS 61.80.Ba; 47.35.+i; 52.38.Mf; 81.15.Fg