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Electric Field Writing of Ferroelectric Nano‐Domains Near 71° Domain Walls with Switchable Interfacial Conductivity
Authors:Shuzhen Yang  Ren‐Ci Peng  Qing He  Yen‐Lin Huang  Yijing Huang  Jan‐Chi Yang  Tianzhe Chen  Jingwen Guo  Long‐Qing Chen  Ying‐Hao Chu  Ce‐Wen Nan  Pu Yu
Institution:1. State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China;2. State Key Lab of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China;3. Department of Physics, Durham University, Durham, UK;4. Department of Materials Science and Engineering, National Chiao Tung University, Hsinchu, Taiwan;5. Department of Physics, National Cheng Kung University, Tainan, Taiwan;6. Department of Materials Science and Engineering, Pennsylvania State University, University Park, PA, USA;7. Collaborative Innovation Center of Quantum Matter, Beijing, China;8. RIKEN Center for Emergent Matter Science, Wako, Japan
Abstract:Conducting ferroelectric domain walls attract a wide range of research interest due to their promising applications in nanoelectronics. In this study, we reveal an unexpected enhanced conductivity near the well‐aligned 71° nonpolar domain walls in BiFeO3. Such an interfacial conductivity is induced by the creation of up‐polarized nano‐domains near the 71° domain walls, as revealed by the combination of the piezo‐response force microscopy (PFM) and conducting atomic force microscopy (c‐AFM) imaging techniques, as well as phase‐field simulations. The upward polarized domains are suggested to lower the Schottky barrier at the interface between the tip and sample surface, and then give rise to the enhanced interfacial conductivity. The result provides a new strategy to tune the local conductance in ferroelectric materials and opens up new opportunities to design novel nanoelectronic devices.
Keywords:domain walls  ferroelectric polarization switching  local conduction  nanodomains
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