Optical line shapes for polymethine dyes and their aggregates: Novel theory of quantum transitions and its correlation with experiment |
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| Authors: | Vladimir V. Egorov |
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| Affiliation: | Russian Academy of Sciences, Photochemistry Center, 7a Novatorov Street, Moscow 119421, Russian Federation |
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| Abstract: | This work reports how a proper theoretical definition of electron-nuclear(-phonon) coupling in the dynamics of the transient state in quantum transitions enables an explanation for the basic experimental data on the optical line shapes for polymethine dyes and their dimers as well as H-, H*-, and J-aggregates, which defied understanding for many decades. |
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| Keywords: | Quantum transitions Dozy chaos Control of dynamics Polymethine dyes Molecular aggregates Optical line shapes |
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