Two-Level Dipolar System in a Heat Bath: High-Pump Power Effects in the Nonlinear Optical Responses |
| |
| Authors: | J. L. Paz J. R. León-Torres Luis Lascano Ysaias J. Alvarado Cesar Costa-Vera |
| |
| Affiliation: | 1.Departamento de Física, Escuela Politécnica Nacional,Quito,Ecuador;2.Departamento de Química,Universidad Simón Bolívar,Caracas,Venezuela;3.Laboratorio de Caracterización Molecular y Biomolecular (LCMB), Centro de Investigaciones y Tecnología de Materiales (CITeMa),Instituto Venezolano de Investigaciones Científicas (IVIC),Miranda,Venezuela;4.Grupo Ecuatoriano para el Estudio Experimental y Teórico de Nanosistemas (GETNano),Diego de Robles y Vía Interoceánica, USFQ,Quito,Ecuador |
| |
| Abstract: | Using the four-wave mixing spectroscopy, we analyze the nonlinear optical properties in a strongly driven two-level system, using a perturbative treatment where, the pump field is considered at all orders, second order in the probe, and first order for the signal field, when the stochastic effects of the solvent are considered. Significant variations in the nonlinear optical properties due mainly to changes in the probe intensity, chemical concentrations, and transversal relaxation times are observed. |
| |
| Keywords: | |
| 本文献已被 SpringerLink 等数据库收录！ |
|
