Investigation of coherence transfer between “CH3” and “CH2” groups in ethanol with time-resolved multiplex CARS technique |
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Authors: | Y.H. Wang X. Du X. He Y.Q. Yang |
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Affiliation: | aCenter for Condensed Matter Science and Technology, Department of Physics, Harbin Institute of Technology, Harbin 150001, China |
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Abstract: | The coherence transfer between stretching vibration modes of C–H bonds in the ethanol is detected by time-resolved multiplex CARS technique and it occurs via “through-bond transfer” pathway. The time scale and velocity of coherence transfer are estimated at 90 fs and 1670 m/s. Moreover, coherence transfer process requires vibrational modes of acceptor and donor are different. |
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Keywords: | Coherence transfer Multiplex CARS |
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