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Investigation of coherence transfer between “CH3” and “CH2” groups in ethanol with time-resolved multiplex CARS technique
Authors:Y.H. Wang   X. Du   X. He  Y.Q. Yang  
Affiliation:aCenter for Condensed Matter Science and Technology, Department of Physics, Harbin Institute of Technology, Harbin 150001, China
Abstract:The coherence transfer between stretching vibration modes of C–H bonds in the ethanol is detected by time-resolved multiplex CARS technique and it occurs via “through-bond transfer” pathway. The time scale and velocity of coherence transfer are estimated at 90 fs and 1670 m/s. Moreover, coherence transfer process requires vibrational modes of acceptor and donor are different.
Keywords:Coherence transfer   Multiplex CARS
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