Phase transformations in highly excited clusters |
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Authors: | A. Chernomoretz and C. O. Dorso |
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Affiliation: | (1) Departamento de Fsica Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón 1 Ciudad Universitaria, 1428 Buenos Aires, Argentina |
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Abstract: | In this communication we analyze the behavior of exciteddrops that undergo fragmentation. We focus our attention on twoscenarios: in the first one the system is free to expand, whilein the second one it is confined inside a spherical volume. Itis shown that the caloric curve of free expanding systems doesnot display a vapor branch. In the case of constrained ones,they behave as undergoing a first order phase transition at lowdensities while as a second order one at high densities. Thetransition from liquid-like to vapor-like behavior is signaledboth by the caloric curves and thermal response functions. |
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Keywords: | 64.60.Qb Nucleation 64.70. Fx Liquid-vaportransitions 31.15.Qg Molecular dynamics and other numericalmethods |
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