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Phase transformations in highly excited clusters
Authors:A. Chernomoretz and C. O. Dorso
Affiliation:(1) Departamento de F"imath"sica Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón 1 Ciudad Universitaria, 1428 Buenos Aires, Argentina
Abstract:In this communication we analyze the behavior of exciteddrops that undergo fragmentation. We focus our attention on twoscenarios: in the first one the system is free to expand, whilein the second one it is confined inside a spherical volume. Itis shown that the caloric curve of free expanding systems doesnot display a vapor branch. In the case of constrained ones,they behave as undergoing a first order phase transition at lowdensities while as a second order one at high densities. Thetransition from liquid-like to vapor-like behavior is signaledboth by the caloric curves and thermal response functions.
Keywords:64.60.Qb Nucleation  64.70. Fx Liquid-vaportransitions  31.15.Qg Molecular dynamics and other numericalmethods
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