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Crystal structure and properties of the uranium chalcogenides α-US2 and α-USe2
Authors:H Noel  JY Le Marouille
Abstract:The uranium chalcogenides α-US2 and α-USe2 crystallize in the tetragonal space group P4ncc and not I4mcm as previously reported. Their crystal structures have been determined from single-crystal X-ray diffraction data and refined to R = 0.041 and R = 0.034, respectively. Uranium atoms occupy two crystallographic sites: U(1) in (8f) and U(2) in (4c). The fourfold position, U(2), is incompletely filled with three uranium atoms which show a significant uniaxial delocalization. Properties are discussed in relation to this new crystal structure.
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