1.Physics Division,Sophia University,Chiyodaku,Japan;2.Graduate School of Science and Engineering,Kagoshima University,Kagoshima,Japan;3.Suzuka National College of Technology,Shiroko-cho Suzuka,Japan
Abstract:
The ground state of the frustrated equilateral triangular spin tube CsCrF4 is still hidden behind a veil though NMR spectrum broaden into 2 T at low temperature. In order to investigate the spin structure in an ordered state by 19F-NMR, we have determined the anisotropic hyperfine coupling tensors for each three fluorine sites in the paramagnetic state. The measurement field was raised up to 10 T to achieve highest resolution. The preliminary analysis using the obtained hyperfine tensors has shown that the archetypal 120°-type structure in ab-plane does not accord with the NMR spectra of ordered state.