| 增强UiO-66-NH2光催化水分解制氢性能的研究进展 |
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| 引用本文： | 王丽苹,李仁星,余莹,阮玉娴,陈琳,姜帅. 增强UiO-66-NH2光催化水分解制氢性能的研究进展[J]. 化学通报, 2024, 87(7): 785-801 |
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| 作者姓名： | 王丽苹 李仁星 余莹 阮玉娴 陈琳 姜帅 |
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| 作者单位： | 曲靖师范学院 化学与环境科学学院,曲靖师范学院 化学与环境科学学院,曲靖师范学院 化学与环境科学学院,曲靖师范学院 化学与环境科学学院,曲靖师范学院 化学与环境科学学院,曲靖市民族中学 |
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| 基金项目： | 云南省地方本科高校基础研究联合专项(202301BA070001-178)、云南省高校绿色催化与能源材料科技创新团队项目、云南省大学生创新创业训练计划项目(S202210684021、S202210684023、S202310684009)、云南省高校协同创新中心(曲靖绿色光伏产业协同创新中心)项目、云南省科技厅科技人才与平台计划项目(202305AF150088)、云南省李和兴专家工作站项目和曲靖市科创企业孵化中心有限公司横向项目资助 |
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| 摘 要： | 氢能是一种能量密度高、储量大、可再生、零污染的新能源。光催化水分解制氢是一种绿色、清洁的能源转换技术，被认为是一种有效的制氢方法。UiO-66-NH2是一种可见光响应、稳定性良好的金属有机骨架材料，但存在可见光响应范围有限、导电性差、载流子复合率高等问题。研究者们采用金属粒子掺杂、染料敏化、金属纳米粒子负载等多种方法对UiO-66-NH2进行改性，提升UiO-66-NH2在光催化水分解制氢反应中的性能，并报道了许多研究成果。因此，本文对近年来报道的有关增强UiO-66-NH2光催化水分解制氢性能的方法进行了综述，并对后续的发展提出了建议，以期为UiO-66-NH2在光催化水分解制氢中应用研究提供参考。
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| 关 键 词： | 氢能，光催化；水分解；UiO-66-NH2 |
| 收稿时间： | 2024-02-02 |
| 修稿时间： | 2024-03-07 |
Progress in improving the properties of UiO-66-NH2 in photocatalytic water splitting for hydrogen production |
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| WANG Liping,RUAN Yuxian,LI Renxing,YU Ying,CHEN Lin and JIANG Shuai. Progress in improving the properties of UiO-66-NH2 in photocatalytic water splitting for hydrogen production[J]. Chemistry, 2024, 87(7): 785-801 |
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| Authors: | WANG Liping RUAN Yuxian LI Renxing YU Ying CHEN Lin JIANG Shuai |
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| Affiliation: | College of chemistry and environmental science,Qujing Normal University,College of chemistry and environmental science,Qujing Normal University,College of chemistry and environmental science,Qujing Normal University,College of chemistry and environmental science,Qujing Normal University,College of chemistry and environmental science,Qujing Normal University,Qujing ethnic mddle school |
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| Abstract: | Hydrogen energy is a new energy source with high energy density, large reserves, renewable energy and zero pollution. Photo-catalytic water splitting for hydrogen production is a green and clean energy conversion technology, which is considered to be an effective hydrogen production method. UiO-66-NH2 is a metal-organic skeleton material with visible light response and good stability. However, it still has the disadvantages of the limited visible light response range, poor conductivity and high recombination of the photo-induced carriers. Many researchers modified UiO-66-NH2 through metal particle doping, dye sensitization, metal nanoparticle loading and other methods to improve the performance of UiO-66-NH2 in the photocatalytic water splitting for hydrogen production and reported many research results. Therefore, in order to provide reference for the further application research of UiO-66-NH2 in photocatalytic water splitting for hydrogen production, the recently reported methods for improving the performance of UiO-66-NH2 in the photocatalytic water splitting for hydrogen production are reviewed, and the suggestions on the subsequent development of the catalysts based on UiO-66-NH2 are put forward. |
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| Keywords: | Hydrogen energy Photocatalysis Water splitting UiO-66-NH2 |
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