Radiochemical measurements of99Tc: Sources and environmental levels |
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| Authors: | E Holm J Rioseco S Ballestra A Walton |
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| Institution: | (1) International Laboratory of Marine Radioactivity, IAEA Oceanographic Museum, (Monaco);(2) Department of Radiation Physics, Lund University, Lund, (Sweden) |
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| Abstract: | A method of99Tc determination has been developed based on sample decomposition followed by purification from interfering elements by hydroxide and oxide precipitations. Technetium is extracted by TBP and electrodeposited onto stainless steel discs from sodium hydroxide solution.99Tcm is used as yield monitor. The method has been applied to study releases from different sources and contents in different samples of atmospheric, terrestrial and marine origin. Results show enhanced99Tc/137Cs activity ratios for samples collected in recent years which are only expected to be contaminated from fallout from nuclear tests. Integrated fallout measurements did not reflect these enhanced ratios. |
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