Influence of the mean free path of reactant particles on the kinetics of diffusion-controlled reactions: Escape probability of geminate recombination |
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| Affiliation: | 1. Hangzhou Institute of Advanced Studies, Zhejiang Normal University, Hangzhou 311231, Zhejiang, China;2. State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, Liaoning, China;3. Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 116023 Dalian, Liaoning, China |
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| Abstract: | The escape probability of geminate particles between which no long-range force acts is calculated as a function of their mean free path. The escape probability increases significantly with an increase in their mean free path, especially when their initial separation is small. |
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