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Graphitic Carbon Nitride Microspheres Supportedα-FeO(OH)Hybrids for Visible Light Photodegradation of MO
作者姓名:WANG Junlin  YI Yongjie  LI Mengjia  CHANG Yue  ZHA Fei
作者单位:College of Chemistry & Chemical Engineering;Key Laboratory of Eco-environment-related Polymer Materials;Key Laboratory of Polymer Material of Gansu Province
基金项目:the National Natural Science Foundation of China
摘    要:Graphitic carbon nitride(g-C3N4)microspheres supported a-FeO(OH)hybridsα-FeO(OH)/g-C3N4]were prepared by means of a self-assembly method in deionized water.By UV-visible diffiise reflectance spectroscopy,it has been confirmed thatα-FeO(OH)/g-C3N4 has a wider absorption range thanThe feature ofα-FeO(OH)/g-C3N4 can be attributed to the efficient separation of the electron-hole pairs with photoluminescence spectra.The degradation rate of methyl orange(MO)is up to 99%under the optimal conditions of 110 min,initial concentration of 30 mg/L,anα-FeO(OH)/g-C3N4 dosage of 15 mg as well as visible light.The mechanism for this photocatalytic reaction was proposed,with hydroxyl radicals being a major active catalytic species.

关 键 词:α-FeO(OH)/g-C3N4  Self-assembly  method  PHOTOCATALYST  Methyl  orange(MO)  Visible  light
收稿时间:2018-06-05

Graphitic Carbon Nitride Microspheres Supported α-FeO(OH) Hybrids for Visible Light Photodegradation of MO
WANG Junlin,YI Yongjie,LI Mengjia,CHANG Yue,ZHA Fei.Graphitic Carbon Nitride Microspheres Supported α-FeO(OH) Hybrids for Visible Light Photodegradation of MO[J].Chemical Research in Chinese University,2019,35(2):319-324.
Authors:WANG Junlin  YI Yongjie  LI Mengjia  CHANG Yue  ZHA Fei
Institution:1. College of Chemistry & Chemical Engineering, Northwest Normal University, Lanzhou 730070, P. R. China;
2. Key Laboratory of Eco-environment-related Polymer Materials, Ministry of Education, Northwest Normal University, Lanzhou 730070, P. R. China;
3. Key Laboratory of Polymer Material of Gansu Province, Northwest Normal University, Lanzhou 730070, P. R. China
Abstract:Graphitic carbon nitride(g-C3N4) microspheres supported α-FeO(OH) hybridsα-FeO(OH)/g-C3N4] were prepared by means of a self-assembly method in deionized water. By UV-visible diffuse reflectance spectroscopy, it has been confirmed that α-FeO(OH)/g-C3N4 has a wider absorption range than g-C3N4. The feature of α-FeO(OH)/g-C3N4 can be attributed to the efficient separation of the electron-hole pairs with photoluminescence spectra. The degradation rate of methyl orange(MO) is up to 99% under the optimal conditions of 110 min, initial concentration of 30 mg/L, an α-FeO(OH)/g-C3N4 dosage of 15 mg as well as visible light. The mechanism for this photocatalytic reaction was proposed, with hydroxyl radicals being a major active catalytic species.
Keywords:α-FeO(OH)/g-C3N4  Self-assembly method  Photocatalyst  Methyl orange(MO)  Visible light  
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