Comparison of linear and 2D IR spectra in the presence of fast exchange |
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Authors: | Kim Yung Sam Hochstrasser Robin M |
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Abstract: | The few picosecond time scale H-bond making and breaking in the system acetonitrile-methanol dominates the mechanism of vibrational coherence transfer that is evident in the shapes of both the linear and nonlinear IR spectra of the CN group. |
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