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纳秒强激光电离苯产生高价碳离子的波长效应
作者单位:中国科学院安徽光学精密机械研究所,合肥,230031;中国科学院研究生院,北京,100039;中国科学院安徽光学精密机械研究所,合肥,230031;中国科学院大连化学物理研究所,大连,116023
基金项目:国家高技术研究发展计划(863计划)
摘    要:

关 键 词:  库仑爆炸  高价原子离子  飞行时间质谱

Wavelength Dependence of Production of Multicharged Carbon Ions in Nanosecond Intense Laser Ionization of Seeded Benzene Beam
Niu Dongmei,Liang Feng,Luo Xiaolin,Wen Lihua,Zhang Xixian,Li Haiyang. Wavelength Dependence of Production of Multicharged Carbon Ions in Nanosecond Intense Laser Ionization of Seeded Benzene Beam[J]. Chinese Journal of Chemical Physics, 2004, 17(4): 375-377. DOI: 10.1088/1674-0068/17/4/375-377
Authors:Niu Dongmei  Liang Feng  Luo Xiaolin  Wen Lihua  Zhang Xixian  Li Haiyang
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Abstract:The photoionization of seeded benzene beam by 25 ns laser pulse at wavelengths of 266,355 and 1064 nm has been studied by the time-of-flight mass spectrometry. The observed mass spectra at 266 nm and 355 nm at intensities of 1010-1011 W/cm2 indicate a multiphoton ionization and dissociation(MPID)process,in which C+,C2Hx+,C3Hx+,C4Hx+ and C6H6+ are main products. While at 1064 nm laser of similar intensities,the domain ion is C4+ which is produced from Coulomb explosion. The longer wavelength facilities the energy absorption rate during inverse bremsstrahlung,which leads to the resulting wavelength dependence of the multicharged atomic ions.
Keywords:Benzene,Coulomb explosion,Multicharged atomic ions,Time of flight mass spectrometry           
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