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Transformations of Isocaryophyllene Diepoxide under Conditions of Homogeneous and Heterogeneous Acid Catalysis
Authors:O V Salomatina  O I Yarovaya  D V Korchagina  Yu V Gatilov  M P Polovinka  V A Barkhash
Institution:(1) Novosibirsk State University, ul. Pirogova 2, Novosibirsk, 630090, Russia;(2) Vorozhtsov Novosibirsk Institute of Organic Chemistry, Siberian Division, Russian Academy of Sciences, pr. Akademika Lavrent'eva 9, Novosibirsk, 630090, Russia
Abstract:Transformations of isocaryophyllene diepoxide (an isomer of widely spread natural sesquiterpene) were studied in various acidic media under conditions of homogeneous and heterogeneous catalysis. A number of previously unknown compounds were thus obtained. The experimental data were compared with the results of molecular-mechanics and quantum-chemical simulation of the most probable transformation paths.
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