Evidence for the preparation of a nonstationary state from the optical double resonance spectrum of NO2 |
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Authors: | HG Weber PJ Brucat RN Zare |
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Institution: | Department of Chemistry, Stanford University, Stanford, California 94305, USA |
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Abstract: | In addition to the narrow resonances from the hyperfine structure of the NO2 excited state, a broad resonance appears in the optical radio frequency double resonance spectrum. It has a pressure-independent linewidth, corresponding to a lifetime of 0.4 ± 0.1 μs, which is attributed to the preparation to the preparation of a nonstationary state by the excitation source. |
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