On the T Bloch law in magnets with fourth-order exchange interaction |
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Authors: | RM Mueller U Köbler K Fischer |
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Institution: | Institut für Festk?rperforschung, Forschungszentrum Jülich, 52425 Jülich, Germany, DE
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Abstract: | For the ferromagnets EuS and GdMg, in which fourth-order exchange interactions (i.e. biquadratic, three-spin and four-spin interactions) have been identified, the deviation of the spontaneous magnetization
with respect to the T
=0 value is shown to follow a T2 law instead of the famous T3/2 law expected for a Heisenberg ferromagnet. Moreover, the observed T2 law holds for temperatures as large as 0.8TC and the extrapolated magnetization value for does not conform to ferromagnetic saturation. This is because the fourth-order exchange interactions generate a second order-parameter
which is assumed to govern the order of the transverse moment components. These moment components have a finite expectation
value for at the expense of the Heisenberg order parameter. Like the spontaneous magnetization, the critical field curves B
c
(
T
) of the metamagnet EuSe and the antiferromagnet EuTe also start decreasing with a T2 term for . It is argued that the T2 law is a consequence of the fourth-order exchange interactions. This is shown experimentally by a study of the critical field
curves 0pt] pertinent to the longitudinal (Heisenberg) order-parameter in the diamagnetically diluted antiferromagnets EuxSr1-xTe. In this solid solution series a particular composition of x
c
=0.85 exists at which the different fourth-order interaction processes compensate each other in the high temperature average. As
a consequence, an EuxSr1-xTe sample with x
=0.85 meets the requirements of a Heisenberg antiferromagnet at least if a quantity is considered for which the high-temperature
average over all fourth-order interactions is decisive. This seems to be the case for the critical field curve 0pt] which
gives the phase boundary to the paramagnetic phase. In fact, a crossover from a T2 to a T3/2 law is observed for 0pt] on approaching xc. This, we believe, shows the frequently observed T2 law is caused by the fourth-order interactions.
Received 23 July 1998 and Received in final form 12 October 1998 |
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Keywords: | PACS 75 30 Et Exchange and superexchange interactions - 75 30 Kz Magnetic phase boundaries (including magnetic transitions metamagnetism etc ) - 75 40 Cx Static properties (order parameter static susceptibility heat capacities critical exponents etc ) |
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