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面向CO2电化学转化的铜基催化剂研究进展
作者单位:
基金项目:the Key Research and Development Project of Tianjin(18ZXJMTG00180);the Key Research and Development Project of Tianjin(19ZXNCGX00030)
摘    要:

关 键 词:二氧化碳  电化学还原  Cu基催化剂  C2+产物  选择性  
收稿时间:2020-06-12

Recent Advances in Electrochemical CO2 Reduction Using Copper-Based Catalysts
Yichen Meng,Siyu Kuang,Hai Liu,Qun Fan,Xinbin Ma,Sheng Zhang. Recent Advances in Electrochemical CO2 Reduction Using Copper-Based Catalysts[J]. Acta Physico-Chimica Sinica, 1985, 37(5): 2006034-0. DOI: 10.3866/PKU.WHXB202006034
Authors:Yichen Meng  Siyu Kuang  Hai Liu  Qun Fan  Xinbin Ma  Sheng Zhang
Affiliation:
Abstract:Burning of fossil fuels increases CO2 concentration in the atmosphere, resulting in a series of climate- and environment-related concerns such as global warming, sea-level rise, and melting of glaciers. Therefore, utilization of renewable energy to reduce the CO2 concentration, in order to realize a sustainable development, is urgent. Capturing and utilizing CO2, a greenhouse gas, can not only address these concerns but also alleviate the current scenario of energy shortage. Thermal catalytic CO2 hydrogenation offers various pathways with high conversion efficiencies to produce fuels and industrial chemicals including CO, HCOOH, CH3OH, and CH4. However, CO2 is chemically inert due to the highly stable C=O bond. Thus, harsh reaction conditions such as high temperature and pressure are required for CO2 hydrogenation.
Keywords:Carbon dioxide  Electrochemical reduction  Copper-based catalysts  C2+ products  Selectivity  
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