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Temperature-dependent electronic structure of gadolinium
Authors:W Nolting  T Dambeck  G Borstel
Institution:(1) Facultad de Ciencias, Fisica Teórica Universidad de Valladolid, E-47011 Valladolid, Spain;(2) Fachbereich Physik, Universität Osnabrück, D-49069 Osnabrück, Germany;(3) Present address: Lehrstuhl Festkörpertheorie, Humboldt-Universität, Invalidenstrasse 110, D-10115 Berlin, Germany
Abstract:We investigate the electronic structure of the ferromagnetic 4f-metal Gadolinium by use of a many-body evaluation of a generalized model of magnetism, the one-particle part of which is derived from an ASW-LSDA bandstructure calculation. A striking temperature-dependence of the conduction band states is traced back to a 4f-(5d, 6s) interband exchange. The conduction electron polarization (0.63 mgr B atT=0) decreases forTrarrT c very similar to the 4f-magnetization. A red shift of the lower uarr-band edge of about 0.25 eV appears upon cooling fromT=T c toT=0. — The quasiparticle band-structure exibits a remarkable non uniform magnetic behaviour at different positions in the Brillouin zone, and in particular for different subbands. Weakly correlated (ldquos-likerdquo) dispersions show a ldquoStoner-likerdquoT-dependence of the exchange splitting. On the other hand, stronger correlated (ldquod-likerdquo) dispersions split belowT c into four branches, two for each spin direction. TheirT-dependence mainly concerns the spectral weights of the quasiparticle peaks and not so much the energetic positions. An exchange caused splitting remains even forT<T c .
Keywords:71  10+x  75  30  Et  75  50  Cc
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