On the origin of the phase–space diffusion limit in (dis)ordered protein aggregation |
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Authors: | A Gadomski J Siódmiak I Santamaría-Holek |
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Institution: | 1. Department of Physics, Institute of Mathematics and Physics, University of Technology and Life Sciences, Kaliskiego 7, 85-796 Bydgoszcz, Poland;2. UMDI-Facultad de Ciencias, Universidad Nacional Autonoma de Mexico, Campus Juriquilla, Queretaro 76230, Mexico |
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Abstract: | Derivation of a phase–space diffusion limit (D-L) allows to obtain a useful formula for a characteristic width of the macroion-channeling filter, controlling model (dis)ordered protein aggregations in a non-ideal aqueous solution. The channel’s width is estimated at the order of an inner half-width of the Stern-type double layer circumventing the growing object and depends in turn on an interplay of the local thermal and electrostatic conditions. The interfacial channeling effect manifests at the edge of biomolecular hydration-duration dependent (non)Markovianity of the system. The interface vs. solution aggregation late-time dynamics are discussed in such local (non)isothermal context with the aim to suggest their experimental assessment. |
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Keywords: | Films Interfaces Crystal Growth |
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