Many-electron effect in the angle resolved L3-M23M23 Auger-photoelectron coincidence spectroscopy (APECS) spectrum of metallic Zn |
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Authors: | Masahide Ohno |
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Institution: | Quantum Science Research 2-8-5 Tokiwadai, Itabashi-ku, Tokyo 174-0071, Japan |
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Abstract: | The many-body effect in the L3-M23M23 Auger-electron spectroscopy (AES) spectrum of metallic Zn is discussed. The lifetime width and residual relaxation energy shift of the two M23-hole state are governed by the (super) Coster-Kronig (sCK) transitions of two M23-hole state. The residual relaxation energy shift and decay width of the two M23-hole state are calculated in an average configuration by an ab initio atomic many-body theory. The agreement with experiment is good. To elucidate the many-body effect in the two-hole states, it is necessary to be able to discriminate individual components of the multiplet-split AES spectrum. We discuss how to discriminate individual components of the multiplet-split L3-M23M23 AES spectrum of metallic Zn by angle-resolved Auger-photoelectron coincidence spectroscopy (AR-APECS) in order to determine accurately their line shapes, multiplet splitting energies, and spin states (singlet etc.). |
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Keywords: | Auger-photoelectron coincidence spectroscopy (APECS) Angle resolved Auger-photoelectron coincidence spectroscopy (AR-APECS) Ab initio atomic many-body theory Lifetime width of two core holes (super) Coster-Kronig transition Zn metal |
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