Metallic ferromagnet with square-lattice CoO2 sheets |
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Authors: | Matsuno J Okimoto Y Fang Z Yu X Z Matsui Y Nagaosa N Kawasaki M Tokura Y |
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Institution: | Correlated Electron Research Center, National Institute of Advanced Industrial Science and Technology, Tsukuba 305-8562, Japan. j-matsuno@aist.go.jp |
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Abstract: | A single-crystalline film of Sr2CoO4 with square-lattice CoO2 sheets (K2NiF4-type structure) was synthesized, and its electronic properties were characterized. The compound exhibited both ferromagnetic and metallic behaviors, with a fairly high Curie temperature T(C) of approximately 250 K, in contrast to the superconductivity recently found in a triangular-lattice CoO2-sheet compound. The film's large magnetoresistance with current perpendicular to the CoO2 plane showed field-hysteretic behavior analogous to tunneling magnetoresistance. The electronic structure of Sr2CoO4 was also investigated to characterize the quasi-two-dimensional ferromagnetic metal state in terms of optical spectroscopy and first-principles calculation. |
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