Förster-type processes in cascading systems |
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Authors: | M. Loher G. Zumofen |
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Affiliation: | Physical Chemistry Laboratory, ETH-Zentrum, CH-8092 Zurich, Switzerland |
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Abstract: | The deactivation of molecules (donors) excited to high vibrational states by consecutively transferring single vibrational quanta to randomly placed acceptors is investigated. Whereas the microscopic master equation is governed by constant step-down rates, the corresponding macroscopic reaction system exhibits not only time-dependent effective rates but also deactivating rates connecting all the levels to each other. |
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