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单分子荧光过程的Monte-Carlo模拟
引用本文:陈宝玖,黄世华.单分子荧光过程的Monte-Carlo模拟[J].发光学报,1998,19(1):14-18.
作者姓名:陈宝玖  黄世华
作者单位:1. 中国科学院长春物理研究所, 长春 130021;2. 中国科学院激发态物理开放研究实验室, 长春 130021
摘    要:从单分子发光过程中电子在激发态上的停留时间t服从P(t)=γe-γt分布出发,对单分子荧光过程进行M-C(Monte-Carlo)随机试验,得到了单分子的激发态相邻两次发光的时间间隔的统计结果以及单分子荧光强度的自相关函数,并对其进行了详细地讨论,这些结果与目前文献报道的实验结果相一致.

关 键 词:单分子荧光  Monte-Carlo模拟  自相关函数
收稿时间:1997-06-09

MONTE CARLO SIMULATION OF THE LUMINESCENCE PROCESS OF SINGLE MOLECULE
Chen Baojiu\ Huang Shihua\ Xu Wu\ Qin Weiping.MONTE CARLO SIMULATION OF THE LUMINESCENCE PROCESS OF SINGLE MOLECULE[J].Chinese Journal of Luminescence,1998,19(1):14-18.
Authors:Chen Baojiu\ Huang Shihua\ Xu Wu\ Qin Weiping
Institution:1. Changchun Institute of Physics, Chinese Academy of Sciences, Changchun 130021;2. Laboratory of Excited State Processes, Chinese Academy of Sciences, Changchun 130021
Abstract:Based on the distribution law P(t)=γe-γt for staying time of single molecule in excited state,this paper simulated the luminescence process of single molecule by Monte Carlo method.The distribution of the time interval between two emission events of a single molecule and the autocorrelation function of the fluorescence intensity were obtained.The simulation features the experimental results reported in the literature recently.
Keywords:luminescence of single molecule  Monte  Carlo simulation  autocorrelation function  
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