Etude des proprietes thermodynamiques et caracterisation des formes allotropiques du soufre condense dans un milieu poreux |
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Authors: | J F Quinson M Brun M Roubin |
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Institution: | (1) Laboratoire de Chimie Appliquée et de Génie Chimique E. R. A. au C. N. R. S n 300, Université Lyon I, 43, Boulevard du 11 Novembre, 1918-69622 Villeurbanne Cedex, France;(2) Laboratoire de Génie Electrique et de Ferroélectricité, Institut National des Sciences Appliquées de Lyon, 20, Avenue Albert Einstein, 69621 Villeurbanne, France;(3) Laboratoire de Chimie Minérale III, Université Lyon 1, 43, Boulevard du 11 Novembre, 1918-69622 Villeurbanne Cedex, France |
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Abstract: | Résumé L'analyse par diffractionX a montré que le soufre retenu dans une matrice mésoporeuse se trouve essentiellement sous la forme orthorhombique et conserve cette structure cristalline jusqu'à la fusion. L'analyse calorimétrique a confirmé pour ce métalloÏde les résultats théoriques régissant le changement d'état liquide solide et a permis d'en déterminer les paramètres: entropie de fusion et énergie interfaciale liquide-solide
ls. Cette étude thermodynamique a montré en outre qu'il était possible de prévoir dans le cas d'un soufre divisé par condensation dans un milieu poreux, une modification du domaine de stabilité des formes allotropiques.
The X-ray analysis of sulphur held in a mesoporous material reveals essentially an orthorhombic crystalline structure. This form does not undergo phase transition before melting.The calorimetric analysis of such a divided sulphur corroborates the theoretical results which were established for liquid solid transformation inside a porous material in a previous paper. Moreover, this analysis helps determine its melting entropy and the solid-liquid surface tension
ls of sulphur.A thermodynamic study also permits a predetermination of the stability range of and allotropic forms in the case of divided sulphur.
Zusammenfassung Die Röntgenanalyse von in halbdurchlÄssigem Material gehaltenem Schwefel zeigt im Wesentlichen eine orthorhombische Kristallstruktur. Diese Form erfÄhrt keinen Phasenübergang vor dem Schmelzen. Die kalorimetrische Analyse eines so verteilten Schwefels erhÄrtete die theoretischen Ergebnisse, welche in einem vorangegangenen Artikel für Flüssigfest-Umwandlungen im Inneren eines porösen Materials dargelegt worden sind. Ausserdem ermöglicht diese Analyse die Schmelz-Entropie und die Festflüssig-OberflÄchenspannung
ls des Schwefels zu bestimmen. Eine thermodynamische Studie gestattet auch die Voraussage zum StabilitÄtsbereich der und allotropischen Formen von verteiltem Schwefel.
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. ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![IOcy](/content/n6m78871725476k5/xxlarge1025.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Mcy](/content/n6m78871725476k5/xxlarge1052.gif) ![IOcy](/content/n6m78871725476k5/xxlarge1025.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Mcy](/content/n6m78871725476k5/xxlarge1052.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![gcy](/content/n6m78871725476k5/xxlarge1075.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![IOcy](/content/n6m78871725476k5/xxlarge1025.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![khcy](/content/n6m78871725476k5/xxlarge1093.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![softcy](/content/n6m78871725476k5/xxlarge1100.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![zhcy](/content/n6m78871725476k5/xxlarge1078.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![kcy](/content/n6m78871725476k5/xxlarge1082.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![softcy](/content/n6m78871725476k5/xxlarge1100.gif) ![gamma](/content/n6m78871725476k5/xxlarge947.gif) . mb. ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) . ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Mcy](/content/n6m78871725476k5/xxlarge1052.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![Mcy](/content/n6m78871725476k5/xxlarge1052.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![CHcy](/content/n6m78871725476k5/xxlarge1063.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![kcy](/content/n6m78871725476k5/xxlarge1082.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![zhcy](/content/n6m78871725476k5/xxlarge1078.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![softcy](/content/n6m78871725476k5/xxlarge1100.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Dcy](/content/n6m78871725476k5/xxlarge1044.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Bcy](/content/n6m78871725476k5/xxlarge1041.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Ucy](/content/n6m78871725476k5/xxlarge1059.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![CHcy](/content/n6m78871725476k5/xxlarge1063.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) ![Vcy](/content/n6m78871725476k5/xxlarge1042.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) - ![Icy](/content/n6m78871725476k5/xxlarge1048.gif) -![Acy](/content/n6m78871725476k5/xxlarge1040.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![lcy](/content/n6m78871725476k5/xxlarge1083.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![pcy](/content/n6m78871725476k5/xxlarge1087.gif) ![Ncy](/content/n6m78871725476k5/xxlarge1053.gif) ![ycy](/content/n6m78871725476k5/xxlarge1099.gif) ![Fcy](/content/n6m78871725476k5/xxlarge1060.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) ![tcy](/content/n6m78871725476k5/xxlarge1090.gif) ![kcy](/content/n6m78871725476k5/xxlarge1082.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![Bcy](/content/n6m78871725476k5/xxlarge1041.gif) ![Ocy](/content/n6m78871725476k5/xxlarge1054.gif) ![scy](/content/n6m78871725476k5/xxlarge1089.gif) ![IEcy](/content/n6m78871725476k5/xxlarge1045.gif) ![Rcy](/content/n6m78871725476k5/xxlarge1056.gif) 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