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Nuclear relaxation studies of the spin-Peierls transition
Authors:LS Smith  E Ehrenfreund  AJ Heeger  LV Interrante  JW Bray  HR Hart  IS Jacobs
Institution:Department of Physics and Laboratory for Research on the Structure of Matter, University of Pennsylvania, Philadelphia, PA 19174, U.S.A.;General Electric Research and Development Center, Schenectady, NY 12301, U.S.A.
Abstract:Nuclear relaxation studies of the spin-Peierls transition in TTF-BDT are presented. At low temperature, but above Tc, the results agree in magnitude, frequency dependence and temperature dependence with calculations based on the pseudofermion treatment of the S = 12, 1-D Heisenberg antiferromagnet. The sharp decrease in the rate below Tc reflects the continuous opening of a magnetic energy gap at the spin-Peierls transition.
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