What is measured in a time-resolved stimulated Raman experiment? |
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Authors: | Martin Van Exter Ad Lagendijk |
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Institution: | Natuurkundig Laboratorium der Universiteit van Amsterdam, Valckenierstraat 65, 1018 XE Amsterdam, The Netherlands |
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Abstract: | We have performed four-beam time-resolved stimulated Raman measurements on liquid CS2. To interpret our results we have applied the response formalism for the third-order polarization to such an experiment. It turns out that the measured quantity is proportional to (a convolution of) Absχ(3)(-ωs, ωs, ωl, -ωl)]. As a consequence in this four-beam e xperiment one picks up electronic contributions in contrast to a two-beam experiment where Imχ(3)] is observed. |
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