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Conversion of CO2 to Multi-carbon Compounds over a CoCO3 Supported Ru-Pt Catalyst Under Mild Conditions
Authors:HUANG Jin  CAI Yichen  YU Yulv  WANG Yuan
Institution:1. Beijing National Laboratory for Molecular Sciences, State Key Lab. for Structural Chemistry of Unstable and Stable Species, College of Chemistry and Molecular Engineering, Peking University, Beijing 100871, P. R. China;2. Sunan Institute for Molecular Engineering, Peking University, Changshu 215500, P. R. China
Abstract:The catalytic hydrogenation of CO2 to multi-carbon compounds under mild conditions would not only provide value-added products, but also benefit for the reduction of CO2 emission if hydrogen derives from renewable energy sources. Herein, we report CoCO3 supported Ru and Pt nano-particles, which could catalyze hydrogenation of CO2 to produce higher hydrocarbons(C2-C26) and higher alcohols(C2OH-C6OH) at low temperatures of 80-130℃. The selectivity for C2+ compounds reached 81.1% at 80℃, which was the highest value reported so far. This work provides a promising catalyst for highly selective converting CO2 and H2 to C2+ compounds at low temperatures.
Keywords:Heterogeneous catalyst  Carbon dioxide  Hydrogenation reaction  Cobalt carbonate  Multi-carbon compound  
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