Magnetic and electrical properties of intercalated phases in the (Cr, Cu)-HfSe2 system |
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Authors: | V G Pleshchev N V Baranov D A Shishkin A V Korolev A D Gorlov |
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Institution: | 1. Gorky Ural State University, ul. Lenina 51, Yekaterinburg, 620083, Russia 2. Institute of Metal Physics, Ural Branch of the Russian Academy of Sciences, ul. S. Kovalevskoi 18, Yekaterinburg, 620990, Russia
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Abstract: | It has been shown that intercalation of the HfSe2 compound with chromium atoms results in an increase in the magnetic susceptibility and a decrease in the resistivity while retaining the semiconductor conductivity type. The Cr x HfSe2 compounds exhibit a paramagnetic behavior at temperatures above 2 K in the entire concentration range 0 ≤ x ≤ 0.25. It has been revealed that an increase in the electron density due to additional introduction of copper can cause the appearance of a cluster-spin-glass-type state in Cr x Cu y HfSe2 compounds. The data obtained indicate a large role of the indirect exchange interaction via conduction electrons in the formation of the magnetic state in layered intercalated compounds based on transition metal dichalcogenides. |
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