VHTR,ADS, and PWR Spent Nuclear Fuel Analysis

The aim of this study is to analyze and compare the discharged-spent fuel of three types of nuclear systems: a Very High-Temperature Gas Reactor (VHTR), a lead-cooled Accelerator-Driven System (ADS) and a standard Pressurized Water Reactor (PWR). The two first systems, VHTR, and ADS were designed to use reprocessed fuels. UREX+ and GANEX techniques were used for the reprocessing processes respectively. The fuel burnup simulated for the systems in other works have been used to obtain the final composition of the spent fuel discharged. After discharge, the radioactivity, the radiotoxicity, and the decay heat were evaluated through the ORIGEN 2.1 code until 10⁷ years and compared to the literature.     

电负性标度与电子亲和能的规律性研究I. 价电子的平均核势

本文将价电子的轨道平均半径~n~l(n、l为轨道的主量子数和角量子数)引入电负性函数中,并采取与常规方法不同的方式确定有效核电荷数Z'。在此基础上,提出新的电负性标度-Z'/~n~l。该标度与Mulliken电负性有良好的线性关系,与Pauling电负性有大体上一致的周期性变化趋势。新标度有一定的物理含义,它代表价电子的平均核势,并且完全可由理论计算得到。