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1.
Five different structures of CH5
+ and one structure of CH5
– are calculated using a gaussian basis both in the SCF approximation and with the inclusion of electron correlation in the independent electron pair approximation (IEPA). While on SCF level the C
sstructure of CH5
+ has to lowest energy, the energy difference between the C
sand C
2vstructures becomes negligible if correlation is included. In contrast to this the approach of a proton to CH4 at large and intermediate distances is most favorable towards a corner of the CH4 tetrahedron which means a structure. The decomposition of CH5
+ into CH3
+ and H2 requires 20kcal/mol on SCF level and 40 kcal/mol if correlation is included. 相似文献
2.
一些实验表明, 实际大气会偏离理想Kolmogorov模型. 本文基于广义Huygens-Fresnel原理和Toselli等提出的非Kolmogorov湍流模型, 推导出部分相干双曲正弦-Gauss (HSG)涡旋光束通过非Kolmogorov大气湍流的解析传输公式, 并用以对两束部分相干HSG涡旋光束相干叠加和非相干叠加形成的合成相干涡旋在非Kolmogorov大气湍流中的动态演化进行了研究. 结果表明, 合成光束平均光强的演化过程与非Kolmogorov湍流的广义指数α, 源平面上叠加涡旋光束拓扑电荷的符号, 以及叠加方式有关. 合成相干涡旋在非Kolmogorov大气湍流中传输时会出现移动、产生和湮灭. 广义指数α, 拓扑电荷符号, 以及叠加方式都会影响其演化行为. 最后, 将本文所得结果与相关文献做了比较. 相似文献
3.
Taking the Gaussian Schell-model pulsed (GSMP) beam as a typical example of spatially and spectrally partially coherent pulsed beams, an analytical expression for the far-field spectrum of diffracted GSMP beams in Young’s interference experiment is derived, and used to study the spectral shifts and spectral switches of GSMP beams in the far field. Numerical calculation results are given to illustrate the dependence of spectral shifts and spectral switches on the obscuration ratio ε, temporal coherent length Tc, spatial correlation parameter β and diffraction angle α. It is shown that the critical angle αc of the first- and second-order spectral switches moves away from the z axis with increasing Tc, but αc of the third-order spectral switch moves towards the z axis with increasing Tc. The spectral transition height Δ decreases and spectral minimum Smin increases as Tc increases. αc decreases, Δ increases and Smin decreases as β increases. The potential application of spectral switches of spatially and spectrally partially coherent pulsed beams in information encoding and transmission is proposed. 相似文献
4.
Influence theory is a foundational theory of physics that is not based on traditional empirically defined concepts, such as positions in space and time, mass, energy, or momentum. Instead, the aim is to derive these concepts, and their empirically determined relationships, from a more primitive model. It is postulated that there exist things, which are call particles, that influence one another in a discrete and directed fashion resulting in a partially ordered set of influence events. The problem of consistent quantification of the influence events is considered. Observers are modeled as particle chains (observer chains) as if an observer were able to track a particle and quantify the influence events that the particle experiences. From these quantified influence events, consistent quantification of the universe of events based on the observer chains is studied. Herein, the kinematics and dynamics of particles from the perspective of influence theory are both reviewed and further developed. 相似文献
5.
We give the formulas of two-pion Hanbury-Brown-Twiss (HBT) correlation function for a partially coherent evolution pion-emitting source, using quantum probability amplitudes in a path-integral formalism. The multiple scattering of the particles in the source is taken into consideration based on Glauber scattering theory. Two-pion interferometry with effects of the multiple scattering and source collective expansion is examined for a partially coherent source of hadronic gas with a finite baryon density and evolving hydrodynamically. We do not find observable effect of either the multiple scattering or the source collective expansion on HBT chaotic parameter. 相似文献
6.
K. Mohammed Jasim 《Optics and Lasers in Engineering》2011,49(7):785-792
The present paper reports an experimental investigation based on X-ray diffraction (XRD), energy dispersive spectroscopy (EDS), and wavelength dispersive spectroscopy (WDS) analyses of phases formed after laser sealing of plasma sprayed coatings of 8.5 wt% yttria partially stabilized zirconia (YPSZ). X-ray diffraction and X-ray step-scanning analyses showed that the plasma sprayed and sealed coatings consisted mainly of t′ phase with a very small amount of monoclinic phase (m phase) in the plasma sprayed coatings. It was also found that the small amounts of m and cubic phases (c phase) present in the sealed coatings were dependent on laser processing specific energies (specific energy is equal to laser power/traverse speed x beam diameter). It was also found that rhombohedral (r) phase formed after laser sealing of coatings at higher specific energies. A direct relationship between c/a ratio of transformable tetragonal phase (t phase) produced by thermal treatment of sealed coatings and nontransformable tetragonal phase (t′ phase) and the amount of Yttria was obtained. A new equation was derived, which describes the relationship between Yttria concentration and the c/a ratio of tetragonal phases (t or t′). 相似文献
7.
8.
9.
LED照明的光栅光调制器光学特性分析与实验 总被引:1,自引:1,他引:1
针对一种新型的光凋制器--光栅光调制器,研究用LED作为其照明光源时对光学调制特性的影响.以部分相干光理论为依据,结合MATLAB仿真,推导出用LED照明光栅光调制器时,光源带宽对成像对比度具有较大的影响,通过滤色片将光源带宽减小到13 nm时,像面上的对比度约为150,进一步减小带宽至10 nm,对比度将达到225.光源的尺寸在与光源到光栅光调制器之间的距离相比小于0.03时,对光栅光调制器的光学信息处理不会有影响,并通过实验加以证实,从而说明采用LED作为光栅光调制器照明光源的可行性. 相似文献
10.
By constructing the recovery operations of the protocol of remote
implementation of partially unknown quantum operation of two qubits
[An-Min Wang: Phys. Rev. A 74 (2006) 032317] with two-qubit Cnot
gate and single qubit logic gates, we present a scheme to implement
it in cavity QED. Long-lived Rydberg atoms are used as qubits, and
the interaction between the atoms and the field of cavity is a
nonresonant one. Finally, we analyze the experimental feasibility of this scheme. 相似文献