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《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2017,129(45):14290-14294
An effective [3+2] annulation tactic for the construction of diverse bicyclic compounds possessing highly functionalized cyclopentane rings has been developed employing soft ketone enolates as the initial nucleophile for anion relay chemistry (ARC). The protocol entails a highly diastereoselective aldol/Brook rearrangement/cyclization cascade. 相似文献
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