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受激拉曼散射(stimulated Raman scattering,SRS)具有激光的特性,并且容易获取不同波长的激光,从而成为调谐激光频率的重要途径之一。然而,由于其转化效率低,限制了它的实际应用。金属纳米粒子具有很强的表面增强效应,曾被广泛地用于增强拉曼散射而获得良好的效果。本文提出将金属纳米粒子的这种性质用于增强SRS。把Au纳米粒子混合于拉曼介质丙酮中,以532nm的纳秒脉冲激光作为激发光,研究了Au纳米粒子在丙酮中的浓度对丙酮SRS一阶Stokes光强的影响,并通过仿真计算对实验结果进行了解释和分析。 相似文献
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Theoretical Analysis of Interference Nanolithography of Surface Plasmon Polaritons without a Match Layer 下载免费PDF全文
Interference nanolithography techniques based on long-range surface plasmon polaritons (LR-SPP) are hardly ever achieved by experiments at present. One key reason is that suitable liquid materials are difflcult to find as the match layer connects the metal film and the resist. We redesign a Kretschmann-Raether structure for interference lithography. A polymer layer is coated under the metal film, and an air layer is placed between the polymer layer and the resist layer. This design not only avoids the above-mentioned question of the match layer, but also can form a soft contact between the polymer layer and the resist layer and can protect the exposure pattern. Simulation results confirm that a device with an appropriately thick polymer layer can form high intensity and contrast interference fringes with a critical dimension of about λ/7 in the resist. In addition, the fabrication of the device is very easy. 相似文献
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This paper describes a multi-reflected mode based on a
narrow waveguide to enlarge the interferential area of surface
plasmon polaritons (SPPs). A reasonable thickness of metal film is
coated under the waveguide, the incident angle and the waveguide
thickness are optimized in order to effectively increase
interferential area. This is a key point for research into the
Goos--H\"anchen shift to optimize the waveguide thickness. Finally,
the SPP interferential field is simulated with the finite-difference
time-domain (FDTD) technique to prove the optimized results, and
indicates that not only is the interferential area enlarged, but
the high contrast is also maintained. Furthermore, the mode can
fabricate some specific interferential patterns by adding some
modulating techniques to the waveguide. So the mode has potential
application in the fabrication of sub-wavelength patterns. 相似文献
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A spatial light modulator (SLM) based on surface plasmon polaritons (SPPs) that can generate chromatic pattern is demonstrated. The device is composed of a waveguide with a thin silver film and an active material. The simulated results show that the SLM can modulate the intensity of three different wavelengths at the same time and combine a colour picture in the image surface. The SLM also owns the characteristics of high sensitivity, high contrast, fast time response etc. This means that the SLM is promising in the chromatic display. 相似文献
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The theoretic analysis of maskless surface plasmon resonant interference lithography by prism coupling 下载免费PDF全文
The use of an attenuated total reflection-coupling mode of prism coated with metal film to excite the interference of the surface plasmon polaritons (SPPs) was proposed for periodic patterning with a resolution of subwavelength scale. High intensity of electric field can be obtained because of the coupling between SPPs and evanescence under a resonance condition, which can reduce exposure time and improve contrast. In this paper, several critical parameters for maskless surface plasmon resonant lithography are described, and the preliminary simulation based on a finite difference timedomain technique agrees well with the theoretical analysis, which demonstrates this scheme and provides the theoretical basis for further experiments. 相似文献
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Surface plasmon polaritons (SPPs) can be excited, meanwhile some peculiar optical phenomena will appear when light irradiates metal structures under some conditions. Based on photonie band gap theory, in this Letter we present a kind of SPP waveguide with multiple wavelength-channels. By using the Bragg effect and introducing some geometric defect layers into a quasi-periodic metal heterowaveguide, the multiple SPP forbidden bands (SPFBs) in a given waveband can be generated, and the multiple SPP pass bands (SPPBs) with narrow bandwidth in each SPFB can be realized. The SPP propagation in metal heterowaveguide is calculated by FDTD and transfer matrix methods. By selecting appropriate thickness, position and the number of defect layers, two SPPBs can be achieved in the SPFBs around 1.31 and 1.55μm simultaneously. 相似文献