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Joseph H. Montoya Kirsten T. Winther Raul A. Flores Thomas Bligaard Jens S. Hummelshj Muratahan Aykol 《Chemical science》2020,11(32):8517
We present an end-to-end computational system for autonomous materials discovery. The system aims for cost-effective optimization in large, high-dimensional search spaces of materials by adopting a sequential, agent-based approach to deciding which experiments to carry out. In choosing next experiments, agents can make use of past knowledge, surrogate models, logic, thermodynamic or other physical constructs, heuristic rules, and different exploration–exploitation strategies. We show a series of examples for (i) how the discovery campaigns for finding materials satisfying a relative stability objective can be simulated to design new agents, and (ii) how those agents can be deployed in real discovery campaigns to control experiments run externally, such as the cloud-based density functional theory simulations in this work. In a sample set of 16 campaigns covering a range of binary and ternary chemistries including metal oxides, phosphides, sulfides and alloys, this autonomous platform found 383 new stable or nearly stable materials with no intervention by the researchers.We present an end-to-end computational system for autonomous materials discovery. 相似文献
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For the specific slip geometry of two sets of coplanar systems (a total of four systems) in fcc metals, the range of dislocation networks in boundaries aligned with one of the two active slip planes is predicted from the Frank equation for boundaries free of long-range elastic stresses. Detailed comparison with experimental data for eight dislocation boundaries in cold-rolled aluminium grains of the 45° ND rotated Cube orientation is conducted. It is concluded that the boundaries are Low-Energy Dislocation Structures, which are in good agreement with the Frank equation while also lowering the energy by dislocation reactions. Cross slip plays a role in the boundary formation process. 相似文献
5.
G. Montagnoli S. Beghini F. Scarlassara A.M. Stefanini L. Corradi C.J. Lin G. Pollarolo Aage Winther 《The European Physical Journal A - Hadrons and Nuclei》2002,15(3):351-356
The two systems 40Ca + 90,96Zr have been studied by measuring nucleon transfer reactions at two energies near the Coulomb barrier, thus complementing
the available sub-barrier fusion cross-sections. Angular distributions for various transfer channels have been determined.
Significantly larger neutron transfer cross-sections are found for the target 96Zr that exhibits the larger enhancement in the sub-barrier fusion cross-sections. All data have been analyzed with a new model
for heavy-ion collisions that calculates simultaneously transfer cross-sections, fusion excitation functions and barrier distributions.
The model gives a good account of both transfer and fusion data.
Received: 2 May 2002 / Accepted: 4 June 2002 / Published online: 26 November 2002
RID="a"
ID="a"e-mail: montagnoli@pd.infn.it, Fax +39049 8277102, Tel. +39049 8277117.
RID="b"
ID="b"On leave from the China Institute for Atomic Energy, 102413 Beijing, China.
Communicated by C. Signorini 相似文献
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A coupled-channel framework for fusion reactions is considered where an ingoing-wave boundary condition allows the effect of strong coupling in the barrier region to be studied. It is shown analytically within the sudden limit and, more generally, with model calculations that the couplings to reaction channels act to enhance the transmission through the barrier at low energies. This appears to be a natural mechanism for explaining the relatively large sub-barrier heavy-ion fusion cross sections which have recently been observed. 相似文献
8.
The paper contains a numerical evaluation of the expressions for the absorptive potential in heavy ion reactions given earlier. With a standard folding expression for the real part of the ion-ion potential general good agreement is found with experimental data for the angular distributions of elastic and inelastic scattering. Special interest is attached to the case of 16O + 28Si where the calculated imaginary potential is very small at low bombarding energies. 相似文献
9.
D. O'Sullivan H. Oestermann P. S. Macmahon L. N. Srivastava J. R. Stubbs N. Mainsbrecq Vivario Stainier M. Schnetka Th. Forgács M. F. Bengen E. Bohm W. Plücker M. Klimmer H. Haupt F. Borchers A. I. Burstein F. S. Frum Orla-Jensen M. O. Winther H. Damen H. A. Sirks Th. v. Fellenberg 《Analytical and bioanalytical chemistry》1936,104(11-12):453-458
10.
A complete local ring of embedding codepth 3 has a minimal free resolution of length 3 over a regular local ring. Such resolutions carry a differential graded algebra structure, based on which one can classify local rings of embedding codepth 3. We give examples of algebra structures that have been conjectured not to occur. 相似文献