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We present high-resolution thermal expansion data from 5-500 K of untwinned YBa2Cu3Ox (Y123) single crystals for x approximately 6.95 and x = 7.0. Large contributions to the thermal expansivities due to O ordering are found for x approximately 6.95, which disappear below a kinetic glasslike transition near 280 K. The kinetics at this glass transition is governed by an energy barrier of 0.98+/-0.07 eV, in very good agreement with other O-ordering studies. Using thermodynamic arguments, we show that O ordering in the Y123 system is particularly sensitive to uniaxial stress along the chain axis and that the lack of well-ordered chains in Nd123 and La123 is most likely a consequence of a chemical-pressure effect. 相似文献
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The thermodynamics of the superconducting transition is studied as a function of doping using high-resolution expansivity data of YBa(2)Cu(3)O (x) single crystals and Monte Carlo simulations of the anisotropic 3D- XY model. We directly show that T(c) of underdoped YBa(2)Cu(3)O (x) is strongly suppressed from its mean-field value (T(MF)(c)) by phase fluctuations of the superconducting order parameter. For overdoped YBa(2)Cu(3)O (x) fluctuation effects are greatly reduced and T(c) approximately T(MF)(c). We find that T(MF)(c) exhibits a similar doping dependence as the pseudogap energy, naturally suggesting that the pseudogap arises from phase-incoherent Cooper pairing. 相似文献
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