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J. Rossat-Mignod P. Burlet T. Kasuya S. Kunii T. Komatsubara 《Solid State Communications》1981,39(3):471-478
Neutron diffraction experiments have been performed on CeB6 single crystals to investigate the magnetic order in zero field. CeB6 orders anti-ferromagnetically below TN = 2.8 ± 0.1 K with a second order phase transition. The magnetic order is defined by the two wave vectors and . No magnetic intensity anomaly has been detected at the transition between the phases II and III. This transition is quite original and corresponds only to a phase shift of the modulation. This unusual behaviour can be understood if the effective Kondo effect is the same in both phases. The structure of the low temperature phase III is probably a helical order in (001) planes with moments along the fourfold axes in constrast with the crystal field anisotropy. In phase III there is a homogeneous moment reduction due to the Kondo effect whereas in the phase II it is non-homogeneous with a sequence (+ μ0 - μ0) containing non-magnetic planes. 相似文献
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The intriguing thermophysical properties of CeB6 have been subject to investigation for more than 20 years. In particular, an exotic ground state, phase IV, emerges under doping with La. We report resonant x-ray scattering results on the order parameter symmetries in phase IV of Ce0.7La0.3B6, which condenses below T(IV)=1.5 K. The results reveal a degree of mesoscopic 5d dipole antiferromagnetic order, with propagation vector Q0=(1/2 1/2 1/2), both below and above T(IV). Below T(IV), this polarization coexists with long-range 4f antiferro-octupole (AFO) order also at Q0. The marked differences in temperature dependence and spatial correlation suggest a state of order parameter segregation at low temperature. A simple model of AFO order, consistent with the polarization dependent azimuth symmetries, the Bragg angle, and temperature dependence is given. 相似文献
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Sera M Ichikawa H Yokoo T Akimitsu J Nishi M Kakurai K Kunii S 《Physical review letters》2001,86(8):1578-1581
The magnetic field induced antiferromagnetic moment M(AF) at low magnetic fields in the antiferroquadrupolar (AFQ) ordered phase of CeB6 was investigated by elastic neutron diffraction experiments for H parallel [110]. The peak intensity at the AF magnetic reciprocal point (1 / 2,1 / 2,1 / 2) corresponding to M(2)(AF) increases with decreasing temperature below the AFQ ordering temperature T(Q), and exhibits a broad maximum at T approximately 3 K and decreases with a further decrease of temperature. This unusual behavior of M(AF) at low fields is explained as a result of the competition between the AF-octupolar and AF-exchange interactions in the O(xy) type AFQ ordered state. 相似文献
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We applied Systematic Evolution of Ligands by EXponential enrichment using Small Cell Lung Cancer (SCLC) cells. A DNA aptamer was identified and evaluated by fluorescent confocal microscopy and flow cytometry. Our results showed that the DNA aptamer binds to molecules that exist predominantly on target SCLC cell surfaces compared with other types of SCLC cells. 相似文献
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Matsumoto J Sugiura Y Yuki D Hayasaka T Goto-Inoue N Zaima N Kunii Y Wada A Yang Q Nishiura K Akatsu H Hori A Hashizume Y Yamamoto T Ikemoto K Setou M Niwa S 《Analytical and bioanalytical chemistry》2011,400(7):1933-1943
Schizophrenia is one of the major psychiatric disorders, and lipids have focused on the important roles in this disorder. In fact, lipids related to various functions in the brain. Previous studies have indicated that phospholipids, particularly ones containing polyunsaturated fatty acyl residues, are deficient in postmortem brains from patients with schizophrenia. However, due to the difficulties in handling human postmortem brains, particularly the large size and complex structures of the human brain, there is little agreement regarding the qualitative and quantitative abnormalities of phospholipids in brains from patients with schizophrenia, particularly if corresponding brain regions are not used. In this study, to overcome these problems, we employed matrix-assisted laser desorption/ionization imaging mass spectrometry (IMS), enabling direct microregion analysis of phospholipids in the postmortem brain of a patient with schizophrenia via brain sections prepared on glass slides. With integration of traditional histochemical examination, we could analyze regions of interest in the brain at the micrometric level. We found abnormal phospholipid distributions within internal brain structures, namely, the frontal cortex and occipital cortex. IMS revealed abnormal distributions of phosphatidylcholine molecular species particularly in the cortical layer of frontal cortex region. In addition, the combined use of liquid chromatography/electrospray ionization tandem mass spectrometry strengthened the capability for identification of numerous lipid molecular species. Our results are expected to further elucidate various metabolic processes in the neural system. 相似文献
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Ryota Shirai Takuya Kunii Akio Yoneyama Takahito Ooizumi Hiroko Maruyama Thet‐Thet Lwin Kazuyuki Hyodo Tohoru Takeda 《Journal of synchrotron radiation》2014,21(4):795-800
Phase‐contrast X‐ray imaging using a crystal X‐ray interferometer can depict the fine structures of biological objects without the use of a contrast agent. To obtain higher image contrast, fixation techniques have been examined with 100% ethanol and the commonly used 10% formalin, since ethanol causes increased density differences against background due to its physical properties and greater dehydration of soft tissue. Histological comparison was also performed. A phase‐contrast X‐ray system was used, fitted with a two‐crystal X‐ray interferometer at 35 keV X‐ray energy. Fine structures, including cortex, tubules in the medulla, and the vessels of ethanol‐fixed kidney could be visualized more clearly than that of formalin‐fixed tissues. In the optical microscopic images, shrinkage of soft tissue and decreased luminal space were observed in ethanol‐fixed kidney; and this change was significantly shown in the cortex and outer stripe of the outer medulla. The ethanol fixation technique enhances image contrast by approximately 2.7–3.2 times in the cortex and the outer stripe of the outer medulla; the effect of shrinkage and the physical effect of ethanol cause an increment of approximately 78% and 22%, respectively. Thus, the ethanol‐fixation technique enables the image contrast to be enhanced in phase‐contrast X‐ray imaging. 相似文献
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H.G. Smith G. Dolling S. Kunii M. Kasaya B. Liu K. Takegahara T. Kasuya T. Goto 《Solid State Communications》1985,53(1):15-19
Lattice dynamics of La11B6 was studied on the neutron triple axis spectrometers at HFIR. The acoustic and optical modes were measured in the high symmetry directions. The rotary motion of the B6 molecule was measured only near the zone boundaries but shows no softening. Instead, very flat low frequency La modes were observed. The agreement with the elastic constants and the temperature dependence of specific heat is satisfactory.In YbB6, the elastic constants and specific heat were measured. Both results give the quite different feature from those of LaB6, no softening of C12 and more softened flat low frequency Yb modes, due to the lack of the metallic bonds. 相似文献
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M. Chiba K. Sera M. Hashizume T. Shimoda S. Sasaki O. Kunii Y. Inaba 《Journal of Radioanalytical and Nuclear Chemistry》2004,259(1):149-152
Environmental conditions were evaluated by element concentrations in hair of children living near the Aral Sea. Hair samples were provided by 63 children living near the Sea (K-district), and 143 children living about 600 km from the Sea (Z-district). PIXE was applied for the determination of elemental concentrations. The concentrations of Br, Na, Hg, and Ni were higher in K-district, and those of Al, Ca, Cr, P, S, and Si were higher in Z-district than in the other district, respectively. It is considered that these results reflect the environmental situation. 相似文献