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钙钛矿太阳能电池(PSCs)成为近几年来迅速发展的新型太阳能电池,其中将SnO2纳米粒子层用作电子传输层(ETL)的钙钛矿太阳能电池器件得到了广泛的关注。SnO2有着更低的制备温度,使其具备应用于柔性器件的潜力,但与钙钛矿层能级不匹配等问题限制着其发展。而在界面处加入钝化层,尤其是表面卤化的方法或可解决这一问题。本文综合研究了SnO2表面卤化对钙钛矿太阳能电池光伏性能的影响,选用四丁基氯化铵(TBAC)、四丁基溴化铵(TBAB)和四丁基碘化铵(TBAI)三种钝化材料对SnO2表面进行钝化处理,并对钝化材料溶液进行了浓度梯度研究。通过材料形貌、结构和光学性能表征以及电池器件性能测试分析等方法,证明了SnO2表面卤化可提高钙钛矿层的质量和PSCs光伏性能,并从器件内部电荷传输动力学等角度解释了器件性能改善的原因。为进一步说明其性能改善的机理,采用基于密度泛函理论(DFT)的第一性原理计算方法对材料表面性质进行了深入研究,从能量、结构、电荷密度、态密度、功函数等角度解释了表面卤化提高SnO2/钙钛矿界面处电子传输特性的原因。实验和理论计算均表明TBAC对于SnO2具有较好的钝化效果,并随着溶液浓度的提升钝化作用越明显。SnO2表面卤化作用的深入研究不仅对提高电池器件性能具有实际意义,还能够帮助理解太阳能电池界面现象,为界面改性提供新的研究思路。 相似文献
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We report a highly efficient three-dimensional degenerated Raman sideband cooling(3D dRSC) that enhances the loading of a magnetically levitated optical dipole trap, and observe the strong atom loss due to the three-body recombination.The 3D dRSC is implemented to obtain 5×107 Cs atoms with the temperature of ~ 480 nK. The cold temperature enables 1.8×107 atoms loaded into a crossed dipole trap with an optimized excessive levitation magnetic gradient. Compared to the loadin... 相似文献
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The centrality dependence of transverse momentum spectra for identified hadrons at midrapidity in Au+Au collisions at √sNN= 200GeV is systematically studied in a quark combination model. The pT spectra of π±, K±, p(p) and Λ(Λ) in different centrality bins and the nuclear modification factors (RCP) for these hadrons are calculated. The centrality dependence of the average collective transverse velocity 〈β(r)〉 for the hot and dense quark matter is obtained in Au+Au collisions, and it is applied to a relative smaller Cu+Cu collision system. The centrality dependence of pT spectra and the RCP for π0, Ks0 and Λ in Cu+Cu collisions at √sNN= 200GeV are well described. The results show that 〈β(r)〉 is only a function of the number of participants Npart and it is independent of the collision system. 相似文献
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We report the generation of heralded single photons with Gaussian-shape temporal waveforms through the spatial light modulation technique in an atomic ensemble. Both the full width at half maximum and the peak position of the Gaussian waveform can be controlled while the single photon nature holds well. We also analyze the bandwidth of the generated single photons in frequency domain and show how the sidebands of the frequency spectrum are modified by the shape of the temporal waveform. The generated single photons are especially suited for the realization of high efficiency quantum storage based on electromagnetically induced transparency. 相似文献
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光导池吸光度表达式的推导与计算──小矩形横截面入射光束 总被引:1,自引:0,他引:1
光导池吸光度表达式的推导与计算──小矩形横截面入射光束刘占军,王云飞(中国科学技术大学应用化学系,合肥,230026)关键词光导池,全反射长毛细管池,吸光度表达式魏磊等[1]分别提出全反射长毛细管池(TR-LCC)中按子午光线和螺旋光线反射行进时的好... 相似文献
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The displacement damage dose methodology for analysing and
modelling the performance of triple-junction InGaP2/GaAs/Ge
solar cells in an electron radiation environment is presented.
Degradations at different electron energies are correlated with
displacement damage dose (D_\rm d). One particular electron
radiation environment, relative to a geosynchronous earth orbit (GEO),
is chosen to calculate the total D_\rm d behind the different
thicknesses coverglasses to predict the performance degradation at
the end of the 15-year mission. 相似文献
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分析了EAST装置偏振干涉仪系统进行电子密度测量时存在的密度跳变信号,开发了密度跳变信号修正程序.结果表明,通过该程序跳变的电子密度数据可以得到有效的修正. 相似文献