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The introduction of mesoporous nanosize zirconia to the catalyst for methanol synthesis dedicates the nanosized catalyst and mesoporous duplicated properties. The catalyst bears the larger surface area, larger mesoporous volume and more uniform diameter, more surface metal atoms and oxygen vacancies than the catalyst prepared with the conventional coprecipitation method. The modification of microstructure and electronic effect could result in the change of the reduced chemical state and decrease of reducuction temperature of copper, donating the higher activity and methanol selectivity to the catalyst. The results of methanol synthesis demonstrate that the Cu^+ is the optimum active site. Also, the interaction between the copper and zirconia shows the synergistic effect to fulfil the methanol synthesis. 相似文献
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Modelling of multi-bodies in close proximity under water waves——Fluid resonance in narrow gaps 总被引:1,自引:0,他引:1
LU Lin TENG Bin CHENG Liang SUN Liang & CHEN XiaoBo Center for Deepwater Engineering Dalian University of Technology Dalian China State Key Laboratory of Structural Analysis for Industrial Equipment State Key Laboratory of Coastal Offshore Engineering School of Civil Resource Engineering The University of Western Australia Crawly Australia Centre for Offshore Research... 《中国科学:物理学 力学 天文学(英文版)》2011,(1)
Viscous fluid model and potential flow model with and without artificial damping force(f=-μV,μ the damping coefficient and V the local averaging flow velocity) are employed in this work to investigate the phenomenon of fluid resonance in narrow gaps between multi-bodies in close proximity under water waves.The numerical results are compared with experimental data available in the literature.The comparison demonstrates that both the viscous fluid model and the potential flow model are able to predict the res... 相似文献
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In this paper a class of iterative methods for the minimax problem i; proposed.We present a sequence of the extented linear-quadratic programming (ELQP) problems as subproblems of the original minimal problem and solve the ELQP problem iteratively.The locally linear and su-perlinear convergence results of the algorithm are established. 相似文献
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The nonconforming Wilson's brick classically is restricted to regular hexahedral meshes. Lesaint and Zlamal[6] relaxed this constraint for the two-dimensional analonue of this element In this paper we extend their results to three dimensions and prove that and where u is the exact solution, u_h is the approximate solution and is the usual norm for the Sobolev space H~1(?). 相似文献
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蒋田仔 《高等学校计算数学学报(英文版)》1997,(2)
This paper deals with the approximate solution of the Fredholm equation Lu= f of the second kind with f ∈H'(Γ). First, we give the order of the n-the optimal radius in the worst case setting. Then, we show that the Galerkin method using 2n+1 inner products of f has minimal error. Finally, we give the estimate of the ε-complexity of the Fredholm problem of the second kind and Galerkin method in the worst case setting. 相似文献
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Bin Gu Hongyuan Liu Yiu-Wing Mai Xi Qiao Feng Shou Wen Yu Centre for Advanced Materials Technology School of Aerospace Mechanical Mechatronic Engineering J University of Sydney Sydney NSW Australia 《Acta Mechanica Sinica》2009,(1)
In the present paper,continuum fracture mecha-nics is used to analyze the Smart-Cut process,a recentlyestablished ion cut technology which enables highly efficientfabrication of various silicon-on-insulator(SOI)wafers ofhigh uniformity in thickness.Using integral transform andCauchy singular integral equation methods,the mode-I andmode-Ⅱ stress intensity factors,energy release rate,and crackopening displacements are derived in order to examine seve-ral important fracture mechanisms involved in the Smart... 相似文献
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ZHU XiaoSong CHENG Liang LU Lin & TENG Bin State Key Laboratory of Coastal Offshore Engineering Dalian University of Technology Dalian China School of Civil Resource Engineering The University of Western Australia Perth WA Australia Centre for Deepwater Engineering Dalian 《中国科学:物理学 力学 天文学(英文版)》2011,(3)
The Moving Particle Semi-implicit (MPS) method performs well in simulating violent free surface flow and hence becomes popular in the area of fluid flow simulation. However, the implementations of searching neighbouring particles and solving the large sparse matrix equations (Poisson-type equation) are very time-consuming. In order to utilize the tremendous power of parallel computation of Graphics Processing Units (GPU), this study has developed a GPU-based MPS model employing the Compute Unified Device Ar... 相似文献
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Yanping Sun Tracey A.Robson Trevor C.BrownSchool of Biological Biomedical & Molecular Sciences University of New England Armidale NSW Australia Manuscript received July revised August 《天然气化学杂志》2002,(Z1)
The oxidative dehydrogenation (ODH) of isobutane over Cr2O3/La2(CO3)3 has been investigated in a low-pressure Knudsen cell reactor, under conditions where the kinetics of the primary reaction steps can be accurately determined. By heating the catalyst at a constant rate from 150-300℃, temperature fluctuations due to non-equilibrium adsorption are minimized. The evolved gas profiles show that ODH to isobutene and water is a primary reaction pathway, while carbon dioxide, which forms from the catalyst during reaction, is the only other product. This CO2 evolution may enhance the activity of the catalyst. Isobutene formation proceeds with the participation of lattice oxygen from the Cr2O3/La2(CO3)3 catalyst. The intrinsic Arrhenius rate constant for the ODH of isobutane isk(s-1) = 1011.5±2.2exp{-((55±5) -ΔHads kJmol-1)/RT}The small pre-exponential factor is expected for a concerted mechanism and for such a catalyst with a small surface area and limited porosity. 相似文献
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