Excellent UV-absorbing cotton fabric with high durability and hydrophobicity based on surface-initiated ATRP of polymerizable organic UV-absorber

Cellulose - Ultraviolet (UV) protective cotton fabric is a convenient and reliable way to protect human body from sunlight. Herein, a polymerizable UV-absorber,...     

基于差异信息量的多源数据融合方法

D-S证据理论可应用于多源数据融合领域，但在处理高度冲突的证据时，可能会出现反直觉的结果.为解决这一问题，本文提出了差异信息量的概念及融合方法.首先，通过信息熵表明证据的相对重要性，采用散度获取证据可信度.然后利用证据可信度优化证据差异度以得到差异信息量，经过计算获取数据的最终权重，并将其作为D-S证据理论中的基本概率分配进行决策.在处理冲突证据、一致证据及不同数量证据等方面的数据融合问题时与其他方法对比，所提方法收敛更快，准确度更高.故障诊断的应用实例表明，所提方法的不确定性更小，优于现存的其他方法.     

Anti-Markovnikov Hydroamination of Racemic Allylic Alcohols to Access Chiral γ-Amino Alcohols

A ruthenium-catalyzed formal anti-Markovnikov hydroamination of allylic alcohols for the synthesis of chiral γ-amino alcohols is presented. Proceeding via an asymmetric hydrogen-borrowing process, the catalysis allows racemic secondary allylic alcohols to react with various amines, affording enantiomerically enriched chiral γ-amino alcohols with broad substrate scope and excellent enantioselectivities (68 examples, up to >99 % ee).     

锂电池异常状态监测的FEKF方法研究

为了保障锂离子电池的使用安全，提出了基于带渐消因子的扩展卡尔曼滤波 （Fading Extended Kalman Filter，FEKF）的电池状态在线监测方法. 建立锂电池一阶等效电路模型，利用递推最小二乘法进行锂电池状态参数在线辨识，建立状态方程；引入最优渐消因子，构造FEKF，得到端电压残差；使用端电压残差序列构造χ2分布的诊断函数，计算误检率与状态参数异常阈值. 实验结果显示利用FEKF生成的残差能更早对异常状态进行告警，证明FEKF能够显著提高χ2检验对锂电池内部缓变型异常状态判断的准确率.     

The Effect of the Spacer of Bis(biurea) Ligands on the Structure of A2L3‐type (A=anion) Phosphate Complexes

By tuning the length and rigidity of the spacer of bis(biurea) ligands L, three structural motifs of the A₂L₃ complexes (A represents anion, here orthophosphate PO₄^3?), namely helicate, mesocate, and mono‐bridged motif, have been assembled by coordination of the ligand to phosphate anion. Crystal structure analysis indicated that in the three complexes, each of the phosphate ions is coordinated by twelve hydrogen bonds from six surrounding urea groups. The anion coordination properties in solution have also been studied. The results further demonstrate the coordination behavior of phosphate ion, which shows strong tendency for coordination saturation and geometrical preference, thus allowing for the assembly of novel anion coordination‐based structures as in transition‐metal complexes.     

Geochemistry of Clayey Aquitard Pore Water as Archive of Paleo-Environment,Western Bohai Bay

The record of paleo-environment in clayey aquitard pore water is much more effective relative to aquifer groundwater owing to the low permeability of clayey aquitard. Oxygen-18 (18O), deuterium (D), an...