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Titration microcalorimetry is used to study the influences of iodide, bromide, and chloride counterions on the aggregation of vesicle-forming 1-methyl-4-(2-pentylheptyl)pyridinium halide surfactants. Formation of vesicles by these surfactants was characterised using transmission electron microscopy. When the counterion is changed at 303 K through the series iodide, bromide, to chloride, the critical vesicular concentration (cvc) increases and the enthalpy of vesicle formation changes from exo- to endothermic. With increase in temperature to 333 K, vesicle formation becomes strongly exothermic. Increasing the temperature leads to a decrease in enthalpy and entropy of vesicle formation for all three surfactants. However the standard Gibbs energy for vesicle formation is, perhaps surprisingly, largely unaffected by an increase in temperature, as a consequence of a compensating change in both standard entropy and standard enthalpy of vesicle formation. Interestingly, standard isobaric heat capacities of vesicle formation are negative, large in magnitude but not strikingly dependent on the counterion. We conclude that the driving force for vesicle formation can be understood in terms of overlap of the thermally labile hydrophobic hydration shells of the alkyl chains. Copyright 2000 Academic Press. 相似文献
3.
de Farias RF de Souza JM de Melo JV Airoldi C 《Journal of colloid and interface science》1999,212(1):123-129
The effects exhibited by adsorbed conducting polyaniline on the redox process on a molybdenum oxide surface were studied. Thermogravimetric results indicate a 4% polyaniline deposition. Cyclic voltammograms of the adsorbed polymer on MoO3 show that polyaniline exerts remarkable effects on the molybdenum blue oxidation-reduction process, with oxidation and reduction potentials of 0.33 and 0.18 V, respectively. This effect strongly enhances the electrode response, and can be used as an important tool in qualitative and/or quantitative determinations of molybdenum in solution as well as in any substrate. Copyright 1999 Academic Press. 相似文献
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Alves GA Amato S Anjos JC Appel JA Astorga J Bracker SB Cremaldi LM Dagenhart WD Darling CL Dixon RL Errede D Fenker HC Gay C Green DR Jedicke R Karchin PE Kennedy C Kwan S Lueking LH de Mello Neto JR Metheny J Milburn RH de Miranda JM da Motta Filho H Napier A Passmore D Rafatian A dos Reis AC Ross WR Santoro AF Sheaff M Souza MH Spalding WJ Stoughton C Streetman ME Summers DJ Takach SF Wallace A Wu Z 《Physical review letters》1996,77(12):2388-2391
7.
Li CK Séguin FH Frenje JA Petrasso RD Delettrez JA McKenty PW Sangster TC Keck RL Soures JM Marshall FJ Meyerhofer DD Goncharov VN Knauer JP Radha PB Regan SP Seka W 《Physical review letters》2004,92(20):205001
Target areal density (rhoR) asymmetries in OMEGA direct-drive spherical implosions are studied. The rms variation / for low-mode-number structure is approximately proportional to the rms variation of on-target laser intensity / with an amplification factor of approximately 1/2(C(r)-1), where C(r) is the capsule convergence ratio. This result has critical implications for future work on the National Ignition Facility as well as OMEGA. 相似文献
8.
Supershell structure in alkali metal nanowires 总被引:1,自引:0,他引:1
Nanowires are formed by indenting and subsequently retracting two pieces of sodium metal. Their cross section gradually reduces upon retraction and the diameters can be obtained from the conductance. In previous work we have demonstrated that when one constructs a histogram of diameters from large numbers of indentation-retraction cycles such histograms show a periodic pattern of stable nanowire diameters due to shell structure in the conductance modes. Here, we report the observation of a modulation of this periodic pattern, in agreement with predictions of a supershell structure. 相似文献
9.
Varnum WS Delamater ND Evans SC Gobby PL Moore JE Wallace JM Watt RG Colvin JD Turner R Glebov V Soures J Stoeckl C 《Physical review letters》2000,84(22):5153-5155
Inertial confinement fusion implosions using capsules with two concentric shells separated by a low density region (double shells) are reported which closely follow one dimensional (1D) radiatively driven hydrodynamics simulations. Capsule designs which mitigate Au M-band radiation asymmetries appear to correspond more closely to 1D simulations than targets lacking mitigation of hohlraum drive M-band nonuniformities. One capsule design achieves over 50% of the unperturbed 1D calculated yield at a convergence ratio of 25.5, comparable to that of a double-shell design for an ignition capsule at the National Ignition Facility. 相似文献
10.
Progress in direct-drive inertial confinement fusion research at the
laboratory for laser energetics
R. L. McCrory D. D. Meyerhofer S. J. Loucks S. Skupsky R. Betti T. R. Boehly T. J.B. Collins R. S. Craxton J. A. Delettrez D. H. Edgell R. Epstein K. A. Fletcher C. Freeman J. A. Frenje V. Yu. Glebov V. N. Goncharov D. R. Harding I. V. Igumenshchev R. L. Keck J. D. Kilkenny J. P. Knauer C. K. Li J. Marciante J. A. Marozas F. J. Marshall A. V. Maximov P. W. McKenty S. F.B. Morse J. Myatt S. Padalino R. D. Petrasso P. B. Radha S. P. Regan T. C. Sangster F. H. Séguin W. Seka V. A. Smalyuk J. M. Soures C. Stoeckl B. Yaakobi J. D. Zuegel 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,44(2):233-238
Direct-drive inertial confinement fusion (ICF) is
expected to demonstrate high gain on the National Ignition Facility (NIF) in
the next decade and is a leading candidate for inertial fusion energy
production. The demonstration of high areal densities in hydrodynamically
scaled cryogenic DT or D2 implosions with neutron yields that are a
significant fraction of the “clean” 1-D predictions will validate the
ignition-equivalent direct-drive target performance on the OMEGA laser at
the Laboratory for Laser Energetics (LLE). This paper highlights the
recent experimental and theoretical progress leading toward achieving this
validation in the next few years.
The NIF will initially be configured for X-ray drive and with no beams
placed at the target equator to provide a symmetric irradiation of a
direct-drive capsule. LLE is developing the “polar-direct-drive” (PDD)
approach that repoints beams toward the target equator. Initial 2-D
simulations have shown ignition. A unique “Saturn-like” plastic ring
around the equator refracts the laser light incident near the equator toward
the target, improving the drive uniformity.
LLE is currently constructing the multibeam, 2.6-kJ/beam, petawatt laser
system OMEGA EP. Integrated fast-ignition experiments, combining the OMEGA
EP and OMEGA Laser Systems, will begin in FY08. 相似文献