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E. V. Sampathkumaran K. Hirota I. Das M. Ishikawa 《Zeitschrift für Physik B Condensed Matter》1993,90(2):195-196
Experimental observations for possible presence of 4f quadrupolar Kondo effect in PrCu2Si2 are critically discussed. A comparison of the low temperature properties of the alloys, Pr
x
Y1–x
Cu2Si2 (x=0.05, 0.2 and 0.4), seems to signal the existence of 4f electric quadrupolar glass phenomenon around 4K forx=0.2. 相似文献
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C.N.R. Rao D.D. Sarma P.R. Sarode E.V. Sampathkumaran L.C. Gupta R. Vijayaraghavan 《Chemical physics letters》1980,76(3):413-415
The valence state of Yb in some of its intermetallics, YbNi2Ge2, YbCu2Si2 and YbPd2Si2 has been investigated by LIII(Yb) absorption edges and X-ray pnotoelectron spectra in the 4f and 4d regions. These studies establish the presence of mixed valence in all three systems and illustrate the utility of 4f and 4d spectra in the study of mixed valence in Yb compounds. 相似文献
4.
The single crystalline form of an insulator, Sr(3)CuIrO(6+delta), is shown to exhibit unexpectedly more than one magnetic transition (at 5 and 19 K) with spin-glass-like magnetic susceptibility behavior. On the basis of this finding, viz., inhomogeneous magnetism in a chemically homogeneous material, we propose that the idea of "phase separation" described for manganites is more widespread in different ways. The observed experimental features enable us to make a comparison with the predictions of a recent toy model on magnetic phase separation in an insulating environment. 相似文献
5.
Maiti K Singh RS Medicherla VR Rayaprol S Sampathkumaran EV 《Physical review letters》2005,95(1):016404
We investigate the origin of charge density wave (CDW) formation in insulators by studying BaIrO3 using high-resolution (1.4 meV) photoemission spectroscopy. The spectra reveal the existence of localized density of states at the Fermi level, E(F), in the vicinity of room temperature. These localized states are found to vanish as the temperature is lowered, thereby, opening a soft gap at E(F), as a consequence of CDW transition. In addition, the energy dependence of the spectral density of states reveals the importance of magnetic interactions, rather than well-known Coulomb repulsion effect, in determining the electronic structure thereby implying a close relationship between ferromagnetism and CDW observed in this compound. Also, Ba core level spectra surprisingly exhibit an unusual behavior prior to CDW transition. 相似文献
6.
E. V. Sampathkumaran I. Das R. Vijayaraghavan A. Hayashi Y. Ueda M. Ishikawa 《Zeitschrift für Physik B Condensed Matter》1993,92(2):191-194
The temperature dependence of the lattice constants of the alloys, RCu2Ge2 (R=Nd, Tb, Dy, Ho and Tm) shows the existence of a lattice strain due to the alignment of the 4f-electric quadrupole at low temperatures. This strain could be related to the deviation of the Néel temperatures (T
N
) from that predicted by de Gennes scaling, thereby indicating the role of the quadrupole on the magnetism. On the other hand, in PrCu2Ge2, for which the enhancement ofT
N
is the largest in thisR series, the lattice constants interestingly behave as if the 4f-quadrupole moment is almost quenched and the anomalous magnetism in this case is attributed to some degree of 4f-delocalisation. 相似文献
7.
G. Wortmann K.H. Frank E.V. Sampathkumaran B. Perscheid G. Schmiester G. Kaindl 《Journal of magnetism and magnetic materials》1985,49(3):325-332
The mean valence of Eu is determined by LIII-edge X-ray absorption (LIII-XA) and 151Eu Mössbauer isomer shift measurementd for the mixed-valent compounds EuPd2Si2 and EuNi2P2 in the temperature range from 1.7 to 300 K. For EuPd2Si2, the behaviour of the satellite line observed in the Mössbauer spectra was investigated in detail. From a comparison of the LIII-Xa and Mössbauer results obtained on identical samples the valence/isomer shift calibration problem as well as possible final-state effects in LIII-XA spectra are discussed. 相似文献
8.
R. Nagarajan A. K. Grover S. K. Dhar P. L. Paulose V. Nagarajan E. V. Sampathkumaran 《Hyperfine Interactions》1988,42(1-4):1227-1230
151Eu Mössbauer studies have been made across the respective superconductive transition temperatures in two compounds, La1.7Eu0.1Sr0.2CuO4?y and EuBa2Cu3O7, having zero resistance state at 25K and 85K respectively. The151Eu isomer shift data establish that Eu ions are in trivalent state at all temperatures. The Mössbauer f-factor does not show any significant anomaly across the TC. 相似文献
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