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Ketteler G Ogletree DF Bluhm H Liu H Hebenstreit EL Salmeron M 《Journal of the American Chemical Society》2005,127(51):18269-18273
Using a photoemission spectroscometer that operates close to ambient conditions of pressure and temperature we have determined the Pd-O phase diagram and the kinetic parameters of phase transformations. We found that on the (111) surface oxidation proceeds by formation of stable and metastable structures. As the chemical potential of O2 increases chemisorbed oxygen forms followed by a thin surface oxide. Bulk oxidation is a two-step process that starts with the metastable growth of the surface oxide into the bulk, followed by a first-order transformation to PdO. 相似文献
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Using scanning tunneling microscopy, we show the phase transition between new structures of NO on Rh(111) in equilibrium with the gas phase near 300 K, in the Torr pressure range. Two phases with (2 x 2) and (3 x 3) periodicity transform into each other as the pressure and temperature change around the equilibrium P-T line. By measuring P and T at coexistence, we determined the heat of adsorption in the (3 x 3) structure. From the phase boundary dynamics, the activation energy barrier between phases were estimated. The results demonstrate that unique information can be obtained from high-pressure and high-temperature studies. 相似文献
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Multiple beam interferometry and video microscopy were used to investigate the layering transition of thin liquid films of 1-undecanol confined between atomically smooth mica surfaces. The expulsion of a molecularly thin lubricant layer was followed directly in two dimensions. Overall, the dynamics of the transition follows theoretical predictions based on two-dimensional hydrodynamics. Frequently, pockets of liquid remain trapped inside the contact area at the end of the transition. The trapped pockets undergo shape transformations to minimize elastic and interfacial energy. 相似文献
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A numerical study of deterministic motion in a random environment in two dimensions is performed. All trajectories are localised except at two isolated points in the parameter space. The distribution of trajectory lengths shows “critical” behaviour as those points are approached. Contact with an analytic estimate, based on analogy with gelation theory, is made in one region of the parameter space. The spatial extent of the trajectories scales with arc length as if they were ideal random walks, surprisingly. 相似文献
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M. C. Abreu M. Alimi C. Baglin A. Baldit G. P. Barreira M. Bedjidian P. Bordalo S. Borenstein J. Britz A. Bussiere P. Busson A. Casaca R. Cases J. Castor C. Charlot B. Chaurand D. Contardo E. Descroix A. Devaux J. Fargeix X. Felgeyrolles P. Force L. Fredj J. M. Gago C. Gerschel P. Gomes P. Gorodetzky J. Y. Grossiord A. Guichard J. P. Guillaud R. Haroutunian L. Kluberg L. Kraus G. Landaud I. Linck C. Louren?o A. Maio L. Peralta M. Pimenta J. R. Pizzi C. Racca S. Ramos A. Romana R. Salmeron A. Sinquin P. Sonderegger J. Varela NA Collaboration 《Zeitschrift fur Physik C Particles and Fields》1988,38(1):129-133
The like-sign dimuons copiously recorded in the NA 38 experiment both inp-U and O?U reactions at 200 GeV/nucleon are interpreted as resulting from decays of π andK mesons in comparable proportions. The ++/?? ratio is large (?1.7) and ascribed to theK + being more copiously produced than theK ?. Both the average transverse momentum and the ++/?? ratio are comparable forp-U and O?U reactions, and both increase only slightly with the transverse energyE T . 相似文献