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The intramolecular and long-range ferromagnetic coupling between p-phenylenediamine radical cations in head-to-tail coupled oligo(1, 4-phenyleneethynylene)s and oligo(1,4-phenylenvinylene)s between neighbors and next-nearest neighbors is described. UV/vis/near-IR experiments show that the radical cations are localized in the pendant p-phenylenediamine units of the conjugated oligomers. The ESR spectra of these oligo(1,4-phenyleneethynylene) and oligo(1, 4-phenylenvinylene) di(radical cation)s are consistent with those of a triplet state. A linear behavior is observed for the doubly integrated ESR intensity of the DeltaM(s) = +/-1 and DeltaM(s) = +/-2 signals with the inverse temperature (I approximately 1/T), consistent with Curie's law. This behavior indicates a triplet ground-state diradical with a large triplet-singlet energy gap or possibly a degeneracy of singlet and triplet states. 相似文献
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George R. Rossman Robert D. Shannon Robert K. Waring 《Journal of solid state chemistry》1981,39(3):277-287
Single-crystal optical absorption spectra of NiO, NiTiO3, NiWO4, NiV2O6, NiNb2O6, Ni2SiO4, Ni3V2O8, LiNiPO4, Li2Ni2Mo3O12, SrNiTeO6, LiScSiO4:Ni, MgSiO3:Ni, and (Mg,Ni)2SiO4 are presented for the purpose of comparing the spectra of yellow and green Ni2+ compounds. Powder spectra of NiTiO3, NiWO4, NiV2O6, NiNb2O6, and Ni3V2O8 in the ultraviolet region help elucidate the more intense charge transfer bands. Bright yellow color results when Ni2+ is in a six-coordinated site significantly distorted from octahedral symmetry. Increased absorption intensity occurs when the metal ion d-d bands are in proximity to an ultraviolet charge transfer band. 相似文献
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Martinez-Diaz MV Rodriguez-Morgade MS Feiters MC van Kan PJ Nolte RJ Stoddart JF Torres T 《Organic letters》2000,2(8):1057-1060
[formula: see text] New unsymmetrically substituted DB24C8-phthalocyanines, which are able to form complexes with suitable dialkylammonium cations, have been prepared. These complexes most probably have a pseudorotaxane geometry. 相似文献
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Francis E. Burstall Udo Hertrich-Jeromin Wayne Rossman 《Comptes Rendus Mathematique》2012,350(7-8):413-416
We show how linear Weingarten surfaces appear as special Ω-surfaces and give a characterization of those linear Weingarten surfaces that allow a Weierstrass type representation. 相似文献