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1.
E. S. Moskalenko M. Larsson K. F. Karlsson P. O. Holtz B. Monemar W. V. Schoenfeld P. M. Petroff 《Physics of the Solid State》2007,49(10):1995-1998
We report on low-temperature microphotoluminescence (μ-PL) measurements of InAs/GaAs quantum dots (QDs) exposed to a lateral
external electric field. It is demonstrated that the QDs’ PL signal could be increased severalfold by altering the external
and/or the internal electric field, which could be changed by an additional infrared laser. A model which accounts for a substantially
faster lateral transport of the photoexcited carriers achieved in an external electric field is employed to explain the observed
effects. The results obtained suggest that the lateral electric fields play a major role for the dot luminescence intensity
measured in our experiment—a finding which could be used to tailor the properties of QD-based optoelectronic applications.
The text was submitted by the authors in English. 相似文献
2.
Björn O. Roos Valera Veryazov Per-Olof Widmark 《Theoretical chemistry accounts》2004,111(2-6):345-351
New basis sets of the atomic natural orbital (ANO) type have been developed for the atoms Li–Fr and Be–Ra. The ANOs have been obtained from the average density matrix of the ground states and the lowest excited states of the atom, the positive ion, and the dimer at its equilibirium geometry. Scalar realtivisitc effects are included through the use of a Douglas–Kroll Hamiltonian. Multiconfigurational wave functions have been used with dynamic correlation included using second-order perturbation theory (CASSCF/CASPT2). The basis sets are applied in calculations of the ground-state potentials for the dimers. Computed bond energies are accurate to within 0.05 eV for the alkaline dimers and 0.02 eV for the alkaline-earth dimers (except for Be2).Acknowledgments.ensp;B.O.R. would like to express his gratitude to Prof. Jacopo Tomasi for all the inspiration that his scientific work has given him through the years and continues to do in particular through the work on solvent effects on molecular properties. This work has been supported by a grant from the Swedish Science Research Council, VR.Contribution to the Jacopo Tomasi Honorary Issue 相似文献
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A two-stage laser ablation process is described, which initially generates a laser-light absorbing image from a conventional photolithographic mask via a UV-flood exposure step. For this purpose a colorless precursor of a dye, i.e., itsleuco form, is imbedded into the polymer to be ablated as a dopant. For poly(methyl methacrylate) as such a polymer, triphenylmethanol, the leuco precursor for the corresponding triphenylmethyl dye represents a good choice for ablation with excimer lasers operating at the wavelength 351 nm. In this fashion conventional masks and exposure tools of UV-photolithography may be used in combination with laser ablation. The resulting images are characterized by a good contrast and reasonably sharp contours. The photochemical mechanism and additional aspects of this two-step process, which resembles the portable conformal mask approach of photolithography, are outlined. 相似文献
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A new C,O-cyclodialkylation of dilithiated cyclic beta-keto esters and beta-keto sulfones with 1,4-dibromo-2-butene is reported which results in regio- and diastereoselective formation of 2-vinyl-2,3,3a,4,5,6-hexahydro-2,3-benzofurans. The products could be efficiently transformed into functionalized bicyclo[3.2.1]octan-8-ones by a palladium-catalyzed rearrangement reaction. In case of sulfone derivatives, this rearrangement proceeds with high stereospecifity to give exclusively the endo-configured diastereomers. The bicyclo[3.2.1]octane skeleton is present in a large number of pharmacologically important natural products. 相似文献
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