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1.
MM. J. Duflos D. Letouz G. Queguiner P. Pastour 《Journal of heterocyclic chemistry》1973,10(6):1083-1084
This communication describes the synthesis of l-methyl-2,3-diformylpyrrole. This new compound is used to prepare a new heterocycle, l-methylcyclohepta[b]pyrrol-6-one and thus allows a new synthesis of l-methylpyrrolo[2,3-d]pyridazine. 相似文献
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Sandberg RL Paul A Raymondson DA Hädrich S Gaudiosi DM Holtsnider J Tobey RI Cohen O Murnane MM Kapteyn HC Song C Miao J Liu Y Salmassi F 《Physical review letters》2007,99(9):098103
We present the first experimental demonstration of lensless diffractive imaging using coherent soft x rays generated by a tabletop soft-x-ray source. A 29 nm high harmonic beam illuminates an object, and the subsequent diffraction is collected on an x-ray CCD camera. High dynamic range diffraction patterns are obtained by taking multiple exposures while blocking small-angle diffraction using beam blocks of varying size. These patterns reconstruct to images with 214 nm resolution. This work demonstrates a practical tabletop lensless microscope that promises to find applications in materials science, nanoscience, and biology. 相似文献
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Pulse compression by use of deformable mirrors 总被引:7,自引:0,他引:7
Zeek E Maginnis K Backus S Russek U Murnane M Mourou G Kapteyn H Vdovin G 《Optics letters》1999,24(7):493-495
An electrostatically deformable, gold-coated, silicon nitride membrane mirror was used as a phase modulator to compress pulses from 92 to 15 fs. Both an iterative genetic algorithm and single-step dispersion compensation based on frequency-resolved optical gating calibration of the mirror were used to compress pulses to within 10% of the transform limit. Frequency-resolved optical gating was used to characterize the pulses and to test the range of the deformable-mirror-based compressor. 相似文献
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Transient birefringence can be induced in a gas of anisotropic molecules by an intense polarized laser pulse. We propose to use this birefringence to phase match nonlinear optical frequency-conversion processes. The conditions for anisotropic phase matching are derived, and experimental conditions required for phase-matched third-harmonic generation in a gas-filled hollow-core fiber are presented. We show that these conditions are experimentally feasible over a significant parameter range, making possible a new type of nonlinear optics. 相似文献
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We demonstrate the use of a deformable-mirror pulse shaper, combined with an evolutionary optimization algorithm, to correct high-order residual phase aberrations in a 1-mJ, 1-kHz, 15-fs laser amplifier. Frequency-resolved optical gating measurements reveal that the output pulse duration of 15.2 fs is within our measurement error of the theoretical transform limit. This technique significantly reduces the pulse duration and the temporal prepulse energy of the pulse while increasing the peak intensity by 26%. It is demonstrated, for what is believed to be the first time, that the problem of pedestals in laser amplifiers can be addressed by spectral-domain correction. 相似文献
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Ranitovic P Tong XM Hogle CW Zhou X Liu Y Toshima N Murnane MM Kapteyn HC 《Physical review letters》2011,106(19):193008
Atoms irradiated with combined femtosecond laser and extreme ultraviolet (XUV) fields ionize through multiphoton processes, even when the energy of the XUV photon is below the ionization potential. However, in the presence of two different XUV photons and an intense laser field, it is possible to induce full electromagnetic transparency. Taking helium as an example, the laser field modifies its electronic structure, while the presence of two different XUV photons and the laser field leads to two distinct ionization pathways that can interfere destructively. This work demonstrates a new approach for coherent control in a regime of highly excited states and strong optical fields. 相似文献