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It is shown that the three pulse stimulated photon echo (3PSE) may be used to determine the yield for intersystem crossing in a guest molecule doped into a host lattice. An exact expression is derived for the intensity of the 3PSE for the case when all three spin sublevels participate in the optical pumping cycle. Yields for intersystem crossing in the systems naphthalene in durene (45%) and pentacene in naphthalene (15%) were obtained from the stimulated photon echo decay. In addition, the 3PSE formation is discussed in pseudo two-level systems where the level structure is caused by magnetic interactions. As an example, the 3PSE decay of the system triphenylmethyl in triphenylamine is analyzed. 相似文献
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Koos Duppen Laurens W. Molenkamp Jos B.W. Morsink Douwe A. Wiersma H.P. Trommsdorff 《Chemical physics letters》1981,84(3):421-424
Optical absorption and picosecond photon echo experiments are used to study the dephasing of pentacene in benzoic acid. It is shown that, while the absorption spectrum of pentacene is effected by proton transfer in the benzoic acid dimer, the dephasing is caused by elastic and inelastic phonon scattering processes. 相似文献
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Simple Zeros of the Riemann Zeta-Function 总被引:1,自引:0,他引:1
Assuming the Riemann Hypothesis, Montgomery showed by meansof his pair correlation method that at least two-thirds of thezeros of Riemann's zeta-function are simple. Later he and Taylorimproved this to 67.25 percent and, more recently, Cheer andGoldston increased the percentage to 67.2753. Here we proveby a new method that if the Riemann and Generalized LindelöofHypotheses hold, then at least 70.3704 percent of the zerosare simple and at least 84.5679 percent are distinct. Our methoduses mean value estimates for various functions defined by Dirichletseries sampled at the zeros of the Riemann zeta-function. 1991Mathematics Subject Classification: 11M26. 相似文献
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Quantum Zeno and anti-Zeno paradoxes 总被引:1,自引:0,他引:1
Continuous observation of a time independent projection operator is known to prevent change of state (the quantum Zeno paradox).
We discuss the recent result that generic continuous measurement of time dependent projection operators will in fact ensure
change of state: an anti-Zeno paradox. 相似文献
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粉粒体两相流的电容层析成象测量 总被引:4,自引:0,他引:4
粉粒体系统中的固相浓度分布的在线测量是十分困难的问题.电容层析成象技术是一种近年来发展起来的非侵入式快速浓度场测量技术.它不干扰流场,不受流动中颗粒浓度、加速度、不透明等因素的制约.本文讨论其测量原理、应用、近期进展、存在的主要问题及其解决的对策. 相似文献